This work describes a process-oriented, microphysical-chemical model to simulate the formation and evolution of aerosols and ice crystals under the conditions prevailing in the upper troposphere and lower stratosphere. The model can be run as a box model or along atmospheric trajectories, and considers mixing, gas phase chemistry 5 of aerosol precursors, binary homogeneous aerosol nucleation, h...

[1] Diamond dust (DD) refers to tiny ice crystals that form frequently in the Polar troposphere under clear sky conditions. They provide surfaces for chemical reactions and scatter light. We have measured the specific surface area (SSA) of DD at Barrow in March–April 2009. We have also measured its chemical composition in mineral and organic ions, dissolved organic carbon (DOC), aldehydes, H2O2...

Bacterially induced carbonate mineralization has been proposed as a new method for the restoration of limestones in historic buildings and monuments. We describe here the formation of calcite crystals by extracellular polymeric substances isolated from Bacillus firmus and Bacillus sphaericus. We isolated bacterial outer structures (glycocalix and parietal polymers), such as exopolysaccharides (...

We study the effect of isoforms of osteopontin (OPN) on the nucleation and growth of crystals from a supersaturated solution of calcium and phosphate ions. Dynamic light scattering is used to monitor the size of the precipitating particles and to provide information about their concentration. At the ion concentrations studied, immediate precipitation was observed in control experiments with no ...

Due to the large natural variability of its microphysical properties, the characterization of solid precipitation is a longstanding problem. Since in situ observations are unavailable in severe convective systems, innovative remote sensing retrievals are needed to extend our understanding of such systems. This study presents a novel technique able to retrieve the density, mass, and effective di...

Gas-liquid-solid phase transition behaviour of water is studied with environmental scanning electron microscopy for the first time. Abnormal phenomena are observed. At a fixed pressure of 450 Pa, with the temperature set to -7 °C, direct desublimation happens, and ice grows continuously along the substrate surface. At 550 Pa, although ice is the stable phase according to the phase diagram, meta...

Bulk microphysical parameterizations that represent mixed-phase processes divide particles into categories such as snow and graupel or hail. The distinction between these is in the primary habit of the particles, where snow is assumed to be unrimed ice crystals or aggregates of crystals that have predominantly grown by deposition of ice, while graupel and hail have grown mostly by collection of...

Abundant glacial geologic evidence present throughout Tibet and the bordering mountains shows that glaciers have oscillated many times throughout the late Quaternary. Yet the timing and extent of glacial advances is still highly debated. Recent studies, however, suggest that glaciation was most extensive prior to the last glacial cycle. Furthermore, these studies show that in many regions of Ti...