Direct mapping of phonon dispersion relations in copper by momentum-resolved x-ray calorimetry.

نویسندگان

  • Ruqing Xu
  • Hawoong Hong
  • Paul Zschack
  • T-C Chiang
چکیده

We have developed a new method of mapping phonon dispersion relations based on momentum-resolved x-ray calorimetry. X-ray scattering intensities are measured at selected points in reciprocal space with suitably chosen polarization configurations; the thermal part of the scattering intensity is extracted by scanning the temperature of the sample. The intensity variations, governed by the phonon populations, are analyzed to yield the energies of the phonons. This method is applied to copper. With high-order effects under control, the results are in excellent agreement with the known phonon dispersion relations.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

نرم شدگی فونون‌های انرژی بالا با گذار عایق - ابررسانا در سیستم ابررسانای Ba1-xKxBiO3

Single crystals of Ba1-xKxBiO3 compound for 0 < x <0.6 from insulator to superconducting region have been grown by electrochemical method. The crystals have been characterized by powder x-ray diffraction and Laue x-ray to determine the crystal structure, formed phases and potassium concentration. Inelastic x-ray scattering spectrum of the crystals has been studied to investigate the phonon pro...

متن کامل

Theory of Nonlinear s-Polarized Phonon-Polaritons in Multilayered Structures

A theory is presented for the dispersion relations of the nonlinear phonon-polaritons arising when phonons are coupled to the electromagnetic waves in multilayered structures of nonlinear materials. The calculations are applied to a multilayered structure consisting of a thin film surrounded by semi-infinite bounding media where each layer may have a frequency dependent dielectric function and ...

متن کامل

Stable atomic structure of NiTi austenite

Nitinol (NiTi), the most widely used shape-memory alloy, exhibits an austenite phase that has yet to be identified. The usually assumed austenitic structure is cubic B2, which has imaginary phonon modes, hence it is unstable. We suggest a stable austenitic structure that " on average " has B2 symmetry (observed by x-ray and neutron diffraction), but it exhibits finite atomic displacements from ...

متن کامل

Fourier-transform inelastic X-ray scattering from time- and momentum-dependent phonon--phonon correlations

The macroscopic characteristics of a material are determined by its elementary excitations, which dictate the response of the system to external stimuli. The spectrum of excitations is related to fluctuations in the density–density correlations and is typically measured through frequency-domain neutron1 or X-ray2–4 scattering. Time-domain measurements of these correlations could yield a more di...

متن کامل

Evaluation of x-ray Brillouin scattering data.

Making use of the classical second-moment sum rule, it is possible to convert a series of constant-Q x-ray Brillouin scattering scans (Q momentum transfer) into a series of constant frequency scans over the measured Q range. The method is applied to literature results for the longitudinal phonon dispersion in several glass formers. The constant frequency scans are well fitted in terms of a Q-in...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Physical review letters

دوره 101 8  شماره 

صفحات  -

تاریخ انتشار 2008