Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers.

نویسندگان

  • S Stern
  • L Holmegaard
  • F Filsinger
  • A Rouzée
  • A Rudenko
  • P Johnsson
  • A V Martin
  • A Barty
  • C Bostedt
  • J Bozek
  • R Coffee
  • S Epp
  • B Erk
  • L Foucar
  • R Hartmann
  • N Kimmel
  • K-U Kühnel
  • J Maurer
  • M Messerschmidt
  • B Rudek
  • D Starodub
  • J Thøgersen
  • G Weidenspointner
  • T A White
  • H Stapelfeldt
  • D Rolles
  • H N Chapman
  • J Küpper
چکیده

We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett.112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.

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عنوان ژورنال:
  • Faraday discussions

دوره 171  شماره 

صفحات  -

تاریخ انتشار 2014