Propagating collective excitations in molten salts

نویسندگان

  • T.Bryk
  • I.Mryglod
چکیده

Longitudinal as well as transverse dynamics of a molten salt beyond the hydrodynamic region is studied within the generalized collective modes (GCM) approach. An analytical three-variable model is applied to the treatment of the coupled longand short-time charge fluctuations. Dispersion laws of propagating kinetic collective excitations such as optic phonon-like modes, heat and shear waves are obtained and analyzed for the case of molten NaCl within the eight-variable GCM scheme, combining the analytical methods and molecular dynamics simulations.

منابع مشابه

Nonhydrodynamic Collective Processes in Molten Salts: Theory and Ab Initio Simulations

We review recent progress in theory and ab initio simulations of collective dynamics in molten salts. Main focus is made on the dispersion of nonhydrodynamic optic-like excitations. A concept of “bare” propagating modes is used for the analysis of polarization effects on the dispersion of longitudinal optic modes. Ab initio molecular dynamics in combination with the generalized modes approach i...

متن کامل

Ab initio study of collective excitations in a disparate mass molten salt.

Ab initio molecular dynamics simulations and the approach of generalized collective modes are applied for calculations of spectra of longitudinal and transverse collective excitations in molten LiBr. Dispersion and damping of low- and high-frequency branches of collective excitations as well as wave-number dependent relaxing modes were calculated. The main mode contributions to partial, total, ...

متن کامل

Molecular dynamics study of the longitudinal modes in disparate-mass binary liquid mixtures.

A series of molecular dynamics simulations of simple liquid binary mixtures of soft spheres with disparate-mass particles were carried out to investigate the origin of the marked differences between the dynamic structure factors of some liquid binary mixtures such as the Li0.7Mg0.3 and Li0.8Pb0.2 alloys. It is shown that the facility for observing peaks associated with fast-propagating modes in...

متن کامل

Collective excitations in molten iron above the melting point: A generalized collective-mode analysis of simulations with embedded-atom potentials

Taras Bryk1,2 and A. B. Belonoshko3 1Institute for Condensed Matter Physics of the National Academy of Sciences of Ukraine, 1 Svientsitskii Street, UA-79011 Lviv, Ukraine 2Institute of Applied Mathematics and Fundamental Sciences, National Technical University of Lviv, UA-79013 Lviv, Ukraine 3Condensed Matter Theory, Department of Theoretical Physics, KTH Royal Institute of Technology, SE-10691...

متن کامل

Collective Excitations in an Early Molten Transition Metal

A. H. Said, H. Sinn, A. Alatas, C. A. Burns, D. L. Price, M. L. Saboungi, W. Schirmacher 5 Argonne National Laboratory, Illinois 60439, U.S.A. Western Michigan University, Kalamazoo, MI, 49008, U.S.A. CRMHT-CNRS 1D avenue de la Recherche Scientifique, 45071 Orléans cedex 2, France CRMD-CNRS 1B rue de la Férollerie 45071 Orléans Cedex 2 France Physik-Dept. E13, Technische Universität München, Ge...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

متن کامل
عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2003