Accuracy of the Hartree-Fock method for Wigner molecules at high magnetic fields
نویسندگان
چکیده
Few-electron systems confined in two-dimensional parabolic quantum dots at high magnetic fields are studied by the Hartree-Fock (HF) and exact diagonalization methods. A generalized multicenter Gaussian basis is proposed in the HF method. A comparison of the HF and exact results allows us to discuss the relevance of the symmetry of the charge density distribution for the accuracy of the HF method. It is shown that the energy estimates obtained with the broken-symmetry HF wave functions become exact in the infinite magnetic-field limit. In this limit the charge density of the broken-symmetry solution can be identified with the classical charge distribution. PACS. 73.20.Qt Electron solids – 73.21.-b Electron states and collective excitations in multilayers, quantum wells, mesoscopic, and nanoscale systems
منابع مشابه
Calculation of Quasi-one-dimensional Interacting Electron Gas Using the Hartree-Fock Method
In this paper, the Hartree-Fock method has been formulated to investigate some of the ground state properties of quasi-one-dimensional interacting electron gas in the presence of the magnetic field. The bare coulomb interaction between electrons has been assumed. For this system, we have also computed some of its thermodynamic and magnetic properties such as the energy, pressure, incompressibil...
متن کاملExact broken-symmetry states and Hartree–Fock solutions for quantum dots at high magnetic fields
Wigner molecules formed at high magnetic fields in circular and elliptic quantum dots are studied by exact diagonalization (ED) and unrestricted Hartree–Fock (UHF) methods with multicenter basis of displaced lowest Landau level wave functions. The broken symmetry states with semi-classical charge density constructed from superpositions of the ED solutions are compared to the UHF results. UHF ov...
متن کاملSpontaneous Symmetry Breaking in Single and Molecular Quantum Dots
Classes of spontaneous symmetry breaking at zero and low magnetic fields in single quantum dots (QD’s) and quantum dot molecules (QDM’s) are discussed in relation to the ratio RW between the interelectron Coulomb repulsion and the harmonic confinement, using spin-and-space unrestricted Hartree-Fock calculations. These include Wigner crystallization for RW . 1, and formation of noncrystallized e...
متن کاملStructures and spectra of gold nanoclusters and quantum dot molecules
Size-evolutions of structural and spectral properties in two types of finite systems are discussed. First we focus on energetics and structures of gold clusters, particularly AuN in the 40.N . 200 range exhibiting a discrete sequence of optimal clusters with a decahedral structural motiff, and on the electronic structure of bare and methyl-thiol passivated Au38 clusters. Subsequently, bonding a...
متن کاملCalculations for Atoms and Diatomic Molecules in Strong Magnetic and Static Electric Fields
Fully numerical mesh solutions of 2D quantum equations of Schrödinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and molecules in strong external fields where neither the external field nor the internal interactions can be considered as a perturbation. The applications of th...
متن کامل