Dynamic polarization in the strong-field ionization of small metal clusters.

نویسندگان

  • Marc Smits
  • C A de Lange
  • Albert Stolow
  • D M Rayner
چکیده

We report on the strong field ionization of small transition metal clusters (nickel, Ni(n) n=1-36) within the quasistatic regime at an infrared wavelength of 1.5 microm and at intensities up to 2 x 10(14) W/cm(2). From ion yields in a constant axial intensity beam, we obtained saturation intensities for the individual Ni(n) clusters. As compared to quasistatic, single active electron calculations, a dramatic suppression of ionization was observed. Dynamic polarization in the laser field likely leads to strong multielectron screening of the "active" electron. Representing the metal clusters as classical conducting spheres, we obtained, via a barrier suppression calculation, the classical ionization rates. Agreement was obtained for larger clusters with n>10 when the dynamic polarization was taken into account, emphasizing the multielectron nature of the ionization suppression.

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عنوان ژورنال:
  • Physical review letters

دوره 93 20  شماره 

صفحات  -

تاریخ انتشار 2004