Measurement of hot electron momentum relaxation times in metals by femtosecond ellipsometry

نویسندگان

  • R. J. Hicken
  • B. J. Hickey
  • B. K. Tanner
چکیده

Time-resolved ellipsometric measurements were made upon Au, Cu, Ag, Ni, Pd, Ti, Zr, and Hf thin films. Using an elliptically polarized pump beam, the decay of the optically induced polarization of the sample was observed. Characteristic relaxation times are extracted and interpreted in terms of scattering of linear and angular momentum of hot electrons. A systematic variation is observed between different metals that reflects their underlying band structure.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Ultrafast quasiparticle relaxation dynamics in normal metals and heavy-fermion materials

We present a detailed theoretical study of the ultrafast quasiparticle relaxation dynamics observed in normal metals and heavy-fermion materials with femtosecond time-resolved optical pump-probe spectroscopy. For normal metals, a nonthermal electron distribution gives rise to a temperature~T! independent electron-phonon relaxation time at low temperatures, in contrast to the T-divergent behavio...

متن کامل

Photoinduced femtosecond relaxation of antiferromagnetic orders in the iron pnictides revealed by ultrafast laser ellipsometry

We report ultrafast softening of the antiferromagnetic order, ~150fs after the electron thermalization, which follows a two-step recovery pathway to reveal a distinct interplay of magnetism and the nematic order in iron pnictides.

متن کامل

Femtosecond Studies of Electron Dynamics at Dielectric-Metal Interfaces

Ultrafast relaxation dynamics of electrons at dielectric-metal interfaces reflect the nature of the electronic interaction with both the substrate and the adsorbed layer. The full understanding of macroscopic electrical transport properties across an interface requires the knowledge of the energies, spatial extent of the interfacial electronic states, and the electron scattering length. With th...

متن کامل

Ultrafast Hot Carrier Dynamics in Materials from Ab Initio Calculations

!!!!!How does an excited electron lose its energy? This problem is central in fields ranging from condensed matter physics to electrical engineering and energy. We developed and applied calculations to study the dynamics of out-of-equilibrium charge carriers – also known as hot carriers (HCs) – in semiconductors and metals [1–3]. We present ab initio calculations of electron-phonon, electron-el...

متن کامل

Impact of electron-impurity scattering on the spin relaxation time in graphene: a first-principles study.

The effect of electron-impurity scattering on momentum and spin relaxation times in graphene is studied by means of relativistic ab initio calculations. Assuming carbon and silicon adatoms as natural impurities in graphene, we are able to simulate fast spin relaxation observed experimentally. We investigate the dependence of the relaxation times on the impurity position and demonstrate that C o...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2005