Exciton energy transfer in pairs of single-walled carbon nanotubes.

نویسندگان

  • Huihong Qian
  • Carsten Georgi
  • Neil Anderson
  • Alexander A Green
  • Mark C Hersam
  • Lukas Novotny
  • Achim Hartschuh
چکیده

We studied the exciton energy transfer in pairs of semiconducting nanotubes using high-resolution optical microscopy and spectroscopy on the nanoscale. Photoluminescence from large band gap nanotubes within bundles is observed with spatially varying intensities due to distance-dependent internanotube transfer. The range of efficient energy transfer is found to be limited to a few nanometers because of competing fast nonradiative relaxation responsible for low photoluminescence quantum yield.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Single Walled Carbon Nanotube Effects on Mixed Convection heat Transfer in an Enclosure: a LBM Approach

The effects of Single Walled Carbon Nanotube (SWCNT) on mixed convection in a cavity are investigated numerically. The problem is studied for different Richardson numbers (0.1-10), volume fractions of nanotubes (0-1%), and aspect ratio of the cavity (0.5-2.5) when the Grashof number is equal to 103. The volume fraction of added nanotubes to Water as base fluid are lowers than 1% to make dilute ...

متن کامل

Direct experimental evidence of exciton-phonon bound states in carbon nanotubes.

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single-walled carbon nanotubes (SWNT) in aqueous suspension. The photoluminescence excitation spectra from several distinct SWNTs show the presence of at least one sideband related to the tangential modes, lying 0.2 eV above the main absorption or emission peak. Both...

متن کامل

Multiple exciton generation by a single photon in single-walled carbon nanotubes.

Multiple-exciton generation in single-walled carbon nanotubes is investigated theoretically. We show that multiple excitons can be directly generated by a single photon through resonant coupling with multiexciton states. Further, the theoretically predicted threshold energy for this process is consistent with recent experimental results. Our calculations clarify the elementary processes of mult...

متن کامل

Theoretical Study on the Chemical Reactivity in the Armchair Single-walled Carbon Nanotube: Proton and Methyl Group Transfer

Proton transfer (PT) and methyl group transfer (MGT) occurring in small biomimetic systems, Formamide-Formamidic acid (FA-FI), and N-formyl-N-methylformamide-(E)-methyl N-formylformimidate (NMFA-NMFI) are investigated in the gas phase and in single-walled carbon nanotubes by using the density functional theory and the ONIOM approach. It is shown that PT reaction is disfavoured in single-walled ...

متن کامل

Suppression of exciton-electron scattering in doped single-walled carbon nanotubes.

We theoretically study the phase relaxation of excitons in doped single-walled carbon nanotubes caused by elastic scattering between an exciton and an electron. Our calculation of the spectral linewidth, that is the inverse of the scattering rate, demonstrates that this dephasing process is unexpectedly suppressed in doped single-walled carbon nanotubes, giving rise to anomalous nonlinear behav...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Nano letters

دوره 8 5  شماره 

صفحات  -

تاریخ انتشار 2008