Satellite-derived estimations of spatial and seasonal variation in tropospheric carbon dioxide mass over China
نویسندگان
چکیده
China has frequently been questioned about the data transparency and accuracy of its energy and emission statistics. Satellite-derived remote sensing data potentially provide a useful tool to study the variation in carbon dioxide (CO2) mass over areas of the earth's surface. In this study, Greenhouse gases Observing SATellite (GOSAT) tropospheric CO2 concentration data and NCEP/NCAR reanalysis tropopause data were integrated to obtain estimates of tropospheric CO2 mass variations over the surface of China. These variations were mapped to show seasonal and spatial patterns with reference to China's provincial areas. The estimates of provincial tropospheric CO2 were related to statistical estimates of CO2 emissions for the provinces and considered with reference to provincial populations and gross regional products (GRP). Tropospheric CO2 masses for the Chinese provinces ranged from 53 ± 1 to 14,470 ± 63 million tonnes were greater for western than for eastern provinces and were primarily a function of provincial land area. Adjusted for land area troposphere CO2 mass was higher for eastern and southern provinces than for western and northern provinces. Tropospheric CO2 mass over China varied with season being highest in July and August and lowest in January and February. The average annual emission from provincial energy statistics of CO2 by China was estimated as 10.3% of the average mass of CO2 in the troposphere over China. The relationship between statistical emissions relative to tropospheric CO2 mass was higher than 20% for developed coastal provinces of China, with Shanghai, Tianjin, and Beijing having exceptionally high percentages. The percentages were generally lower than 10% for western inland provinces. Provincial estimates of emissions of CO2 were significantly positively related to provincial populations and gross regional products (GRP) when the values for the provincial municipalities Shanghai, Tianjin, and Beijing were excluded from the linear regressions. An increase in provincial GRP per person was related to a curvilinear increase in CO2 emissions, this being particularly marked for Beijing, Tianjin, and especially Shanghai. The absence of detection of specific elevation of CO2 mass in the troposphere above these municipalities may relate to the rapid mixing and dispersal of CO2 emissions or the proportion of the depth of the troposphere sensed by GOSAT.
منابع مشابه
Trend Spatial & Temporal Distribution, and Sources of the Tropospheric So2 over China Based on Satellite Measurement during 2004~2009
Administration (LRCVES/CMA), National Satellite Meteorological Center, China Meteorological Administration, Beijing 100081,China (2) State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC), The Institute of Atmospheric Physics, CAS, Beijing 100029, China (3) Belgian Institute for Space Aeronomy (BIRA-IASB), Brussels, Belgium ABSTRACT In this study, SCIAMACHY/...
متن کاملSpatiotemporal variations of tropospheric SO2 over China by SCIAMACHY observations during 2004-2009
This paper presents results of measurements of tropospheric sulphur dioxide (SO2) from satellite over China during 2004e2009. SCIAMACHY/ENVISAT SO2 data products have been validated by ground based remote sensing instrument MAXDOAS in China, and with predictions of the atmospheric model GEOSeChem. The spatial and temporal distribution of tropospheric SO2 over China is discussed in this study. T...
متن کاملThe global chemistry transport model TM5: description and evaluation of the tropospheric chemistry version 3.0
We present a comprehensive description and benchmark evaluation of the tropospheric chemistry version of the global chemistry transport model TM5 (Tracer Model 5, version TM5-chem-v3.0). A full description is given concerning the photochemical mechanism, the interaction with aerosol, the treatment of the stratosphere, the wet and dry deposition parameterizations, and the applied emissions. We e...
متن کاملStudy of tropospheric ozone concentration trend of Kermanshah by meteorological parameter and ozone precursor and OMI images
Abstract: Clean air is a necessity for human well-being and health. Air pollution is a major threat to humans and other organisms and is considered as one of the environmental challenges. Today, with the increase in air pollution, the need to know more about the causes of its occurrence has been raised. The various consequences of air pollution have made air quality monitoring and control inev...
متن کاملEstimation of Satellite-Based SO42- and NH4+ Composition of Ambient Fine Particulate Matter over China Using Chemical Transport Model
Epidemiologic and health impact studies have examined the chemical composition of ambient PM2.5 in China but have been constrained by the paucity of long-term ground measurements. Using the GEOS-Chem chemical transport model and satellite-derived PM2.5 data, sulfate and ammonium levels were estimated over China from 2004 to 2014. A comparison of the satellite-estimated dataset with model simula...
متن کامل