Two-Dimensional Electronic Spectroscopy Using Incoherent Light: Theoretical Analysis

Observation of Electronic Excitation Transfer through Light Harvesting Complex II Using Two-dimensional Electronic-vibrational Spectroscopy.

Light Harvesting Complex II (LHCII) serves a central role in light harvesting for oxygenic photosynthesis, and is arguably the most important photosynthetic antenna complex. In this work, we present two-dimensional electronic-vibrational (2DEV) spectra of LHCII isolated from spinach, demonstrating the possibility of using this technique to track the transfer of electronic excitation energy betw...

The effect of incoherent ultraviolet light on the renal capsule tissue using dynamic mechanical analysis and FTIR spectroscopy

Center Line Slope Analysis in Two-Dimensional Electronic Spectroscopy

Center line slope (CLS) analysis in 2D infrared spectroscopy has been extensively used to extract frequency-frequency correlation functions of vibrational transitions. We apply this concept to 2D electronic spectroscopy, where CLS is a measure of electronic gap fluctuations. The two domains, infrared and electronic, possess differences: In the infrared, the frequency fluctuations are classical,...

Two-Dimensional Electronic Spectroscopy of the Low-Light Adapted Light Harvesting Complex 4

Two-dimensional electronic spectroscopy of Light Harvesting Complex 4 from photosynthetic bacteria reveals excited state dynamics on two timescales and resolves exciton states with little to no oscillator strength. The results suggest a molecular structure in which the pigment dipole organization within the circular complex has more tangential than radial character.

Two-dimensional crystals: spectroscopy and electronic applications

The success in creating atomically thin and mechanically robust two-dimensional (2D) crystals, starting with graphene, has unveiled new possibilities for next generation of ultrafast and ubiquitous electronics. One critical distinction between 2D crystals and 3D crystals is that 2D crystals are all-surface materials. Therefore, it is essential to understand how 2D materials interact with their ...