منابع مشابه
Time-resolved photoemission on the attosecond scale: opportunities and challenges.
The interaction of laser pulses of sub-femtosecond duration with matter opened up the opportunity to explore electronic processes on their natural time scale. One central conceptual question posed by the observation of photoemission in real time is whether the ejection of the photoelectron wavepacket occurs instantaneously, or whether the response time to photoabsorption is finite leading to a ...
متن کاملTime-Resolved Two-Photon Photoemission at Metal–Dielectric Interfaces
We review the influence of rare-gas layers on image-potential states at metal surfaces. Experiments on Xe, Kr, and Ar on Cu(100) and on Xe/Ru(0001) that use the technique of time-resolved two-photon photoemission are discussed. The energetic position of the electron affinity, the geometry of the adsorbate layer, and dielectric screening are the factors that influence the dynamical and energetic...
متن کاملTime-resolved photoemission of correlated electrons driven out of equilibrium
B. Moritz,1,2 T. P. Devereaux,1,3 and J. K. Freericks4 1Stanford Institute for Materials and Energy Science (SIMES), SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA 2Department of Physics and Astrophysics, University of North Dakota, Grand Forks, North Dakota 58202, USA 3Geballe Laboratory for Advanced Materials, Stanford University, Stanford, California 94305, USA 4Depa...
متن کاملMeasuring correlated electron dynamics with time-resolved photoemission spectroscopy
Time-resolved photoemission experiments can reveal fascinating quantum dynamics of correlated electrons. However, the thermalization of the electronic system is typically so fast that very short probe pulses are necessary to resolve the time evolution of the quantum state, and this leads to poor energy resolution due to the energy-time uncertainty relation. Although the photoemission intensity ...
متن کاملGauge invariance in the theoretical description of time-resolved angle-resolved pump/probe photoemission spectroscopy
Nonequilibrium calculations in the presence of an electric field are usually performed in a gauge, and need to be transformed to reveal the gauge-invariant observables. In this work, we discuss the issue of gauge invariance in the context of time-resolved angle-resolved pump/probe photoemission. If the probe is applied while the pump is still on, one must ensure that the calculations of the obs...
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ژورنال
عنوان ژورنال: Physical Review B
سال: 2016
ISSN: 2469-9950,2469-9969
DOI: 10.1103/physrevb.93.241114