Review on multi-scale models of solid-electrolyte interphase formation
نویسندگان
چکیده
منابع مشابه
Electrolyte and Solid-Electrolyte Interphase Layer in Lithium-Ion Batteries
The supply and the management of the energy are particularly at the centre of our daily concerns and represent a socio-economic priority. Indeed, while cars use fossil fuel as the main source of energy for over a century, the depletion of the oil reserves and the necessity to reduce the carbon dioxide emissions, stimulate the development of electric vehicles. Therefore, one of the main challeng...
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Aiming at an improved knowledge of the formation of the solid electrolyte interphase (SEI), as basis for the safe and efficient use of new anode materials, we investigated the SEI formation on silicon and lithium titanate (LTO) anodes by electrochemical impedance spectroscopy (EIS) and ex situ X-ray photoelectron spectroscopy (XPS) measurements. While the EIS measurements performed at equidista...
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Aqueous lithium energy storage systems address environmental sustainability and safety issues. However, significant capacity fading after repeated cycles of charge-discharge and during float charge limit their practical application compared to their nonaqueous counterparts. We introduce an artificial solid electrolyte interphase (SEI) to the aqueous systems and report the use of graphene films ...
متن کاملHow Solid-Electrolyte Interphase Forms in Aqueous Electrolytes.
Solid-electrolyte interphase (SEI) is the key component that enables all advanced electrochemical devices, the best representative of which is Li-ion battery (LIB). It kinetically stabilizes electrolytes at potentials far beyond their thermodynamic stability limits, so that cell reactions could proceed reversibly. Its ad hoc chemistry and formation mechanism has been a topic under intensive inv...
متن کاملAb initio molecular dynamics simulations of the initial stages of solid-electrolyte interphase formation on lithium ion battery graphitic anodes.
The decomposition of ethylene carbonate (EC) during the initial growth of solid-electrolyte interphase (SEI) films at the solvent-graphitic anode interface is critical to lithium ion battery operations. Ab initio molecular dynamics simulations of explicit liquid EC/graphite interfaces are conducted to study these electrochemical reactions. We show that carbon edge terminations are crucial at th...
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ژورنال
عنوان ژورنال: Current Opinion in Electrochemistry
سال: 2019
ISSN: 2451-9103
DOI: 10.1016/j.coelec.2018.10.013