Improved Simulations of Global Black Carbon Distributions by Modifying Wet Scavenging Processes in Convective and Mixed?Phase Clouds
نویسندگان
چکیده
In-cloud wet scavenging dominates the removal of aerosols in atmosphere, but is not well represented climate models. Aircraft measurements black carbon (BC) concentrations suggest that models commonly overestimate BC upper troposphere tropics by more than one order magnitude underestimate burdens polar latitudes. In this study, we improved in-cloud parameterizations for convective clouds and mixed-phase to better characterize abundances remote atmosphere (remote oceans regions) with a global model, CAM5-ATRAS2. The modified processes model achieved realistic simulation over both Arctic. new, unified scheme vertical transport during deep convection generally reproduced observed low mixing ratios (about 0.1 ng kg?1) middle tropics, Wegener–Bergeron–Findeisen process (WBF) lowered efficiency from consequently increased Arctic about factor 2. direct radiative forcings 20% globally (from 0.26 0.31 W m?2), importantly 2 0.09 0.18 m?2). Our results indicated good agreement between modeled could be obtained without requiring relatively short lifetime (?4 days) suggested previous studies.
منابع مشابه
Global-mean precipitation and black carbon in AR4 simulations
[1] How much and why precipitation changes as the climate warms is uncertain, even for the global mean. In the 21st Century of the IPCC AR4 A1b forcing scenario, globalmean precipitation increase per degree warming varies among models by over a factor of three. Clear-sky atmospheric shortwave absorption change explains over half of the intermodel spread (r = 0.61) in precipitation increase. Rem...
متن کاملRedistribution of trace gases by convective clouds – mixed-phase processes
The efficiency of gas transport to the free and upper troposphere in convective clouds is investigated in an axisymmetric dynamic cloud model with detailed microphysics. In particular, we examine the sensitivity of gas transport to the treatment of gas uptake by different ice hydrometeors. Two parameters are used to describe this uptake. The gas retention coefficient defines the fraction of dis...
متن کاملGlobal soil carbon projections are improved by modelling microbial processes
Society relies on Earth system models (ESMs) to project future climate and carbon cycle feedbacks. However, the soil C response to climate change is highly uncertain in these models1,2 and they omit key biogeochemical mechanisms3–5. Specifically, the traditional approach in ESMs lacks direct microbial control over soil C dynamics6–8. Thus, we tested a new model that explicitly represents microb...
متن کاملScavenging of black carbon in mixed phase clouds at the high alpine site Jungfraujoch
1 Laboratory for Atmospheric Chemistry, Paul Scherrer Institut, 5232 Villigen PSI, Switzerland 2 Leibniz-Institute for Tropospheric Research, 04318 Leipzig, Germany 3 School of Earth, Atmospheric and Environmental Sciences, University of Manchester, M60 1QD, UK 4 Institute for Atmospheric Physics, German Aerospace Centre, 82234 Wessling, Germany * now at: Institute for Atmospheric and Climate S...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Journal Of Geophysical Research: Atmospheres
سال: 2021
ISSN: ['2169-8996', '2169-897X']
DOI: https://doi.org/10.1029/2020jd033890