Direct conversion of methane to zeolite-templated carbons, light hydrocarbons, and hydrogen
نویسندگان
چکیده
Efficient direct valorization of methane to value-added chemicals and materials remains an unsolved challenge for modern chemistry science. In this work, we explored non-oxidative conversion hydrogen, hydrocarbons, valuable zeolite-templated carbon materials. First, using a set spectroscopy microscopy characterization tools, investigated how the reaction conditions influence process formation inside typical zeolite-based catalyst Mo/ZSM-5. Then, effect zeolite topology on growth from decomposition over Mo/MFI, Mo/MOR, Mo/BEA, Mo/FAU templates. Finally, applied obtained insights prepare high-quality carbons directly Fe/BEA Fe/FAU Altogether, our results represent carbon-economic method COx-free hydrogen gas, mixture light aliphatic aromatic
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ژورنال
عنوان ژورنال: Carbon
سال: 2023
ISSN: ['0008-6223', '1873-3891']
DOI: https://doi.org/10.1016/j.carbon.2022.09.050