Crystal structure of 4-{[l-(4-dimethylaminophenyI)methylidene]amino} · 1,5-dimethyl-2-phenyl-1,2-dihydropyrazol-3-one, C20H22N4O

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Crystal structure of 4-[(E)-(4-hy­droxy­benzyl­idene)amino]-1,5-dimethyl-2-phenyl-1H-pyrazol-3(2H)-one

The asymmetric unit of the title compound, C18H17N3O2, comprises three independent mol-ecules (1, 2 and 3). In mol-ecule 1, the dihedral angles between the pyrazolone ring and the pendant phenyl and hydroxybenzene rings are 54.43 (6) and 28.72 (6)°, respectively. The corresponding data for mol-ecule 2 are 86.84 (6) and 25.69 (5)°, respectively, and for mol-ecule 3 are 47.41 (7) and 17.09 (7)°, ...

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Crystal structure of 4-[[(1E)-(2-hydroxynaphthyl)methylidene]amino]-1,5-dimethyl-2-phenyl-2,3-dihydro-1H-pyrazol-3-one.

bonds [either N–H···O (keto-amine tautomer) or N···H–O (phenol-imine tautomer)] can exist. It is claimed that the hydrogen-bond type depends neither on the stereochemistry of the molecule nor on the sort of substituent bonded to the N imino atom, but on the kind of aldehyde used.1 In the solid state, it is also claimed that only an intramolecular N–H···O type hydrogen bond is present in naphtha...

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(E)-4-(4-Hydr­oxy-3-nitro­benzyl­idene­amino)-1,5-dimethyl-2-phenyl-1H-pyrazol-3(2H)-one

In the title compound, C(18)H(16)N(4)O(4), the dihedral angles between the central pyrazole ring and the pendant substituted and unsubstituted aromatic rings are 4.73 (12) and 44.24 (14)°, respectively. An intra-molecular O-H⋯O hydrogen bond occurs. In the crystal structure, an inter-molecular C-H⋯O inter-action may help to consolidate the packing and a short intra-molecular C-H⋯O contact also ...

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(E)-1,5-Dimethyl-4-[3-(4-nitro­benz­yloxy)benzyl­ideneamino]-2-phenyl-1H-pyrazol-3(2H)-one

In the title compound, C(25)H(22)N(4)O(4), the central benzene ring, makes dihedral angles of 74.35 (6), 17.01 (8) and 62.19 (7)°, respectively, with the nitro-benzyl ring, the pyrazolone ring and the terminal phenyl ring. Inter-molecular C-H⋯O hydrogen bonds help to consolidate the crystal packing.

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4-{(E)-[2-(4-Iodo­but­oxy)benzyl­idene]amino}-1,5-dimethyl-2-phenyl-1H-pyrazol-3(2H)-one

The title Schiff base compound, C(22)H(24)IN(3)O(2), adopts an E configuration about the central C=N bond. The pyrazolone ring makes a dihedral angle of 49.68 (10)° with its attached phenyl ring. The phenolate plane makes dihedral angles of 16.78 (9) and 50.54 (9)°, respectively, with the pyrazolone ring and the terminal phenyl ring. An intra-molecular C-H⋯O hydrogen bond generates an S(6) ring...

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ژورنال

عنوان ژورنال: Zeitschrift für Kristallographie - New Crystal Structures

سال: 2005

ISSN: 2197-4578,1433-7266

DOI: 10.1524/ncrs.2005.220.14.273