Battery impedance spectrum prediction from partial charging voltage curve by machine learning

نویسندگان

چکیده

Electrochemical impedance spectroscopy (EIS) is an effective technique for Lithium-ion battery state of health diagnosis, and the spectrum prediction by charging curve expected to enable testing during vehicle operation. However, mechanistic relationship between curves remains unclear, which hinders development as well optimization EIS-based techniques. In this paper, we predicted voltage optimized input based on electrochemical analysis machine learning. The internal relationships curve, incremental capacity are explored, improves physical interpretability helps define proper partial range learning models. Different algorithms have been adopted verification proposed framework sequence-to-sequence predictions. addition, predictions with different ranges, at charge, training data ratio evaluated prove method high generalization robustness. experimental results show that has accuracy converges findings analysis. errors less than 1.9 mΩ selected corelative reactions inside batteries. Even reduced 3.65–3.75 V, still reliable most RMSEs 4 mΩ.

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ژورنال

عنوان ژورنال: Journal of Energy Chemistry

سال: 2023

ISSN: ['2096-885X', '2095-4956']

DOI: https://doi.org/10.1016/j.jechem.2023.01.004