Acoustothermal Nucleation of Surface Nanobubbles
نویسندگان
چکیده
Ultrasonic surface vibration at high frequencies (O(100 GHz)) can nucleate bubbles in a liquid within few nanometres from surface, but the underlying mechanism and role of wettability remain poorly understood. Here, we employ molecular simulations to study characterize this phenomenon, which call acoustothermal nucleation. We observe that nanobubbles on both hydrophilic hydrophobic surfaces, energy balances are used identify whether these boiling or cavitation events. rationalize nucleation events by defining physics-based balance, matches our simulation results. To interplay between acoustic parameters, wettability, mechanism, produce regime map nanoscopic connects observed nanoscale results macroscopic experiments. This work provides insights better design range industrial processes clinical procedures such as treatments, mass spectroscopy, selective cell destruction.
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ژورنال
عنوان ژورنال: Nano Letters
سال: 2021
ISSN: ['1530-6992', '1530-6984']
DOI: https://doi.org/10.1021/acs.nanolett.0c03895