Nuclear accidents that lead to melting of a reactor core create heterogeneous materials containing hundreds of radionuclides, many with short half-lives. The long-lived fission products and transuranium elements within damaged fuel remain a concern for millennia. Currently, accurate fundamental models for the prediction of release rates of radionuclides from fuel, especially in contact with wat...

An acceptable long-term solution for used (spent) fuel from nuclear power reactors has evaded all countries engaged in the civilian nuclear fuel cycle. Furthermore, many countries are trying to develop interim storage solutions that address the shortage of storage in the spent fuel cooling pools at reactors. The United States has a particularly acute problem due to its adherence to an open fuel...

A review of the chemistry occurring inside a nuclear power plant during a serious reactor accident is presented. This includes some aspects of the behavior of nuclear fuel, its cladding, cesium and iodine. This review concentrates on the chemistry of an accident in a water-cooled reactor loaded with uranium dioxide or mixed metal oxide fuel. Subjects: Chemistry; Environmental Chemistry; Inorgan...

With growing demands for commercial nuclear power, there is also a growing need for better energy efficiency from nuclear power reactors. In order to reach a high burnup up to 100 MWd/kg, previous research has examined the use of thorium-plutonium mixedoxide fuel as a potential candidate for this high-burnup goal. Though the neutronics studies have looked upon this fuel type favorably, the purp...