[1] A global three-dimensional model of tropospheric chemistry driven by reanalyzed European Centre for Medium-Range Weather Forecasts meteorological data is used to examine the sources of O3, CO, and nitrogen oxides (NOx = NO + NO2) in the South Pacific troposphere during the NASA Pacific Exploratory Mission to the Tropics (PEMTropics A) in September–October 1996. Aircraft observations up to 1...

We analyze detailed atmospheric gas/aerosol composition data acquired during the 2008 NASA ARCTAS (Arctic Research of the Composition of the Troposphere from Aircraft and Satellites) airborne campaign performed at high northern latitudes in spring (ARCTAS-A) and summer (ARCTAS-B) and in California in summer (ARCTAS-CARB). Biomass burning influences were widespread throughout the ARCTAS campaign...

Recent observational analysis reveals the central role of three multicloud types, congestus, stratiform, and deep convective cumulus clouds, in the dynamics of large-scale convectively coupled Kelvin waves, westward-propagating two-day waves, and the Madden–Julian oscillation. A systematic model convective parameterization highlighting the dynamic role of the three cloud types is developed here...

This paper examines the influence of imposed drying, intended to represent horizontal advection of dry air, on parameterized deep convection interacting with large-scale dynamics in a single-column model framework. Two single-column models, one based on the NASA Goddard Earth Observing System general circulation model version 5 (GEOS5) and the other developed by Bony and Emanuel, are run in wea...

In this analysis, Tropospheric Emission Spectrometer (TES) V004 nadir ozone (O3) profiles are validated with more than 4400 coinciding ozonesonde measurements taken across the world from the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) during the period 2005–2010. The TES observation operator was applied to the sonde data to ensure a consistent comparison between TES and ozonesonde...

Using a combination of ozonesonde data and numerical simulations of the Chemical Lagrangian Model of the Stratosphere (CLaMS), the trend of tropospheric ozone (O3) during 2002–2010 over Beijing was investigated. Tropospheric ozone over Beijing shows a winter minimum and a broad summer maximum with a clear positive trend in the maximum summer ozone concentration over the last decade. The observe...

The influence of clouds on the large-scale atmospheric circulation is examined in numerical simulations from an atmospheric general circulation model run with and without atmospheric cloud radiative effects (ACRE). In the extratropics of both hemispheres, the primary impacts of ACRE on the circulation include 1) increases in the meridional temperature gradient and decreases in static stability ...

The ozone variability observed by tropospheric ozone lidars during the ESCOMPTE campaign is analyzed by means of a hybrid-Lagrangian modeling study. Transport processes responsible for the formation of ozone-rich layers are identified using a semi-Lagrangian analysis of mesoscale simulations to identify the planetary boundary layer (PBL) footprint in the free troposphere. High ozone concentrati...

[1] The meteorological mechanisms for lofting trace gases and aerosols out of the planetary boundary layer (PBL) into the free troposphere are key to understanding local air pollution problems as well as regional and global atmospheric chemistry and climate issues. Over the North American continent, convective storms and lifting in warm conveyor belts transport pollutants into the free troposph...

An algorithm has been developed that retrieves water vapour profiles in the upper troposphere and lower stratosphere from optical depth spectra obtained by the Measurements of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (MAESTRO) instrument onboard the SCISAT satellite as part of the Atmospheric Chemistry Experiment (ACE) mission. The retrieval relies on ro-v...