The optical properties of molecules dissolved in glasses and ligated to proteins are very similar. The technique of three pulse stimulated photon echo peak shift is used to explore these properties. For dilute chromophores in a glass, a model of linear coupling to a harmonic bath combined with temperature-independent inhomogeneous broadening works well from 30 to 300 K. For concentrated chromop...

We investigate the equilibrium unfolding of Zn-cytochrome c in guanidine hydrochloride by three-pulse photon echo peak shift (3PEPS) spectroscopy. Unexpectedly, the measurements reveal that inhomogeneous broadening of the sample at the midpoint of the denaturation is larger than that of either native or unfolded states. To interpret this finding, we present simulations of the peak shift for bot...

We have measured the shape of the Autler–Townes doublet and the peak of electromagnetically induced transparency (EIT) under plasma conditions. We compare the experimental results with the calculated spectrum of the probe field of a three-level ArII Λ-scheme by taking into account Coulomb collisions. We show that the Coulomb broadening of the EIT peak is small (less than 40%), while the saturat...

Reflection electron energy loss spectra from some insulating materials (CaCO3, Li2CO3, and SiO2) taken at relatively high incoming electron energies (5-40 keV) are analyzed. Here, one is bulk sensitive and a well-defined onset of inelastic excitations is observed from which one can infer the value of the band gap. An estimate of the band gap was obtained by fitting the spectra with a procedure ...

Spectral narrowing of nearly chirp-free 50-fs pulses delivered by a diode-pumped ytterbium solid-state laser (Yb DPSSL) is experimentally demonstrated using an anomalously dispersive, highly nonlinear photonic-crystal fiber (PCF). The ratio of spectral narrowing and the accompanying temporal pulse broadening are controlled by the peak power of Yb DPSSL pulses at the input of the fiber.

Dispersion in spectral domain optical coherence tomography (SD OCT) system cause a degradation of point spread function (peak broadening) after FFT of the spectrum with the increase of the optical path distance between an object and reference arm. Different sources of dispersion and methods for the compensation are shown.

We report supercontinuum (SC) generation centered on the telecommunication C-band (1550 nm) in CMOS compatible hydrogenated amorphous silicon waveguides. A broadening of more than 550 nm is obtained in 1cm long waveguides of different widths using as pump picosecond pulses with on chip peak power as low as 4 W.

The 3 ps pulses are amplified to ~20 GW peak power in a TEA CO(2) laser using ac Stark broadening. Demonstration of such broadband coherent amplification of 10 μm pulses opens opportunities for a powerful mid-IR source at a high-repetition rate.