in the first part of this work, correlation between optical activity and elements of magnetic susceptibility tensor (mst) for five classes of model small molecules containing a single chiral center has been studied using quantum computational techniques at dft-b3lyp level of theory with 6-311g basis set. several molecular properties are used to reduce the mst elements prior to the examination o...

We exploit theoretically a magneto-controlled nonlinear optical material which contains ferromagnetic nanoparticles with a non-magnetic metallic nonlinear shell in a host fluid. Such an optical material can have anisotropic linear and nonlinear optical properties and a giant enhancement of nonlinearity, as well as an attractive figure of merit. Electronic address: [email protected] 1 Fi...

We propose and systematically investigate a novel tunable, compact room temperature terahertz (THz) source based on difference frequency generation in a hybrid optical and THz micro-ring resonator. We describe detailed design steps of the source capable of generating THz wave in 0.5-10 THz with a tunability resolution of 0.05 THz by using high second order optical susceptibility (χ((2))) in cry...

The optical second-harmonic generation SHG and the linear optical properties were investigated in a planar cell containing aligned nonchiral nematic derivative of B10H10 : 14-heptyloxypyridin-1-yl -104-pentyl-1-thiacyclohexyl -closo-decaborane HPTD as a function of temperature. The compound showed a low level of the SHG signal in the polycrystalline state, and no nonlinear optical effect was de...

Mid-infrared (MIR) sideband generation on a near infrared (NIR) optical carrier is demonstrated within a quantum cascade laser (QCL). By employing an externally injected NIR beam, E(NIR), that is resonant with the interband transitions of the quantum wells in the QCL, the nonlinear susceptibility is enhanced, leading to both frequency mixing and sideband generation. A GaAs-based MIR QCL (E(QCL)...

The nonlinear optical properties of plasmon resonant metamaterials consisting of chains of metal nanoparticles are evaluated. Introducing particle size differences along the chains leads to the development of cascaded plasmon resonances exhibiting increased field enhancement and field confinement. The interplay among the different resonances on the structures induces a frequency-dependent enhan...

We investigate the color-locked twin-noisy-field correlation effects in third-order nonlinear absorption and dispersion of ultrafast polarization beats. We demonstrate a phase-sensitive method for studying the twophoton nondegenerate four-wave mixing NDFWM due to atomic coherence in a multilevel system. The reference signal is another one-photon degenerate four-wave-mixing signal, which propaga...

We present a brief overview of different methods for simultaneous phase-matching of several parametric optical processes (the so-called multistep cascading) in engineered structures with the modulated second-order nonlinear susceptibility. In particular, we discuss the possibility of double phase-matching in both uniform and non-uniform quasi-phase-matched (QPM) periodic optical superlattices a...

2014 Optical nonlinear properties of semiconducting organic polymers with one dimensional 03C0 electron system are described. The third order nonlinear susceptibility of these polymers is specially high (#10-10 esu) and their time response very short (~ 1 ps ). Three and two photon resonances due to even and odd parity excited states are observed by third harmonic generation (THG) and by electr...

We present an analytical theory for the nonlinear optical response of a strongly interacting Rydberg gas under conditions of electromagnetically induced transparency. Simple formulas for the third-order optical susceptibility are derived and shown to be in excellent agreement with recent experiments. The obtained expressions reveal strong nonlinearities, which in addition are of highly nonlocal...