The spinel oxides Zn0.4Co0.6AlxFe2-xO4 (x=0.0, 0.25, 0.50, 0.75 & 1.0) have been synthesized in the solid state sintering process in air. X-ray diffraction measurements have been carried out in order to check the phase which showed single phase spinel structure for all the samples. Initial permeability, frequency dependence of the complex permeability sintered at different temperatures has been...