A technique of computing the pressure drop and deposition rate evolution during soot loading and the 3D distribution of deposited soot particles for micro-structured ceramic filter media is presented. Methods developed at Fraunhofer ITWM for generating 3D computer models representing the microstructure of the filter material and for computing soot particle deposition in the microstructure model...

Slightly soluble atmospherically relevant organic compounds may influence particle CCN activity and therefore cloud formation. Adipic acid is a frequently employed surrogate for such slightly soluble organic materials. The 11 published experimental studies on the CCN activity of adipic acid particles are not consistent with each other nor do they, in most cases, agree with the Köhler theory. Th...

This paper examines the incremental global climate response of black carbon (BC), the main component of soot, due to absorption and scattering by BC inclusions within cloud and precipitation particles. Modeled soot is emitted as an externally mixed aerosol particle. It evolves to an internal mixture through condensation, hydration, dissolution, dissociation, crystallization, aqueous chemistry, ...

The present study is concerned with measuring and simulating soot formation and combustion in turbulent liquid fuel spray flames. Soot concentrations inside the combustor are measured by filter paper technique. The simulation is based on the solution of the fully-coupled conservation equations for turbulent flow, chemical species kinetic modeling, fuel droplet evaporation and combustion and...

Number fractions of externally mixed particles of four different sizes (30, 50, 80, and 150 nm in diameter) were measured using a Volatility Tandem DMA. The system was operated in a street canyon (Eisenbahnstrasse, EI) and at an urban background site (Institute for Tropospheric Research, IfT), both in the city of Leipzig, Germany as well as at a rural site (Melpitz (ME), a village near Leipzig)...

The main objective of the work presented in this paper will be to present and discuss the development and implementation of a numerical model to simulate soot formation and depletion in turbulent diffusion flames. The relevance of such model lays on the importance of tying the formation of soot to the ongoing reaction mechanism so that it is fully integrated into the combustion process. The mod...

In this article we present a parameter free aggregation model for soot formation. Each soot particle is represented as a fractal aggregate that can be described by its total volume, total surface, and number of hydrogenated sites on its surface. The moments of the joint Probility Density Function (PDF) of these three quantities are solved using the Direct Quadrature Method of Moments (DQMOM). T...

Introduction To date there are still many unknowns on how particles are formed from gas phase reactive systems such as combustion. It is possible to study particles in-situ using X-ray scattering techniques: Separate applications have shown that the size distribution of soot particle can be measured using Small-Angle X-ray Scattering (SAXS) [1-4] and particle structure with Wide-Angle X-ray Sca...