The analysis of soot formation and oxidation is essential for Diesel engine development to meet future pollutant emission reduction requirements. In recent years laser-induced incandescence (LII) has developed to a powerful tool for soot diagnostics in flames, even in the challenging environment of Diesel combustion. This work presents some recent applications of LII for soot particle sizing in...

The formation of polycyclic aromatic hydrocarbons (PAH) and soot has become one of the central themes of research activities in the area of combustion and pyrolysis of hydrocarbon fuels. The interest in the subject stems mostly from environmental concerns on pollutant emission from combustion devices. The research activities span experimental, theoretical, and computational efforts and cover a ...

The soot formation processes of conventional and low temperature diesel combustion were investigated by a newly developed Forward Illumination Light Extinction (FILE) soot measurement technique in a constant volume spray chamber. The FILE technique has the capability to obtain two-dimensional time-resolved quantitative soot measurements. For diesel combustion at conventional ambient condition, ...

This paper presents an advanced version of the original software developed by the author in order to simulate the combustion in the Diesel engines, focusing on simulate soot formation. Complex kinetic mechanisms are need for realistic modeling of shoot formations, but this is applicable only for simple flame computations (e.g. one dimensional, laminar, etc.). For real turbulent flame calculatio...

A CFD-based numerical model has been developed for the determination of the volume concentration and number density of soot in a laminar diffusion flame of methane in air, under transient condition following ignition of the flame. The transience is studied from the point of ignition till the final steady state is reached. The burner is an axi-symmetric co-flowing one with the fuel issuing throu...

Soot volume fraction and number density in a turbulent diffusion flame burning kerosene/air were predicted using two approaches. The first used a conventional soot inception model based on the acetylene concentration and is referred to as the acetylene model. The second used a soot inception model based on the formation rate of three and two ring aromatics [1] and is referred to as the PAH ince...

In this article we present a parameter free aggregation model for soot formation. Each soot particle is represented as a fractal aggregate that can be described by its total volume, total surface, and number of hydrogenated sites on its surface. The moments of the joint Probility Density Function (PDF) of these three quantities are solved using the Direct Quadrature Method of Moments (DQMOM). T...

While emissions of pollutants from conventional sources, such as industrial and thermal processes, have been in decline over the last two decades, fires have become major sources for the emission of several contaminants. This review summarises chemical mechanisms pertinent to the formation of prominent pollutants, such as NOx, HCN, HCl, soot, and trace species, such as PCDD/Fs (dioxins). We com...

Closed-cage all-carbon molecules referred to as fullerenes were discovered in carbon vapor from laser heating of graphite and subsequently produced in macroscopic quantities by resistive heating of carbon rods. Suggestions that fullerenes may be involved in soot formation, and the detection, in flames, of all-carbon ions having the same masses as fullerenes, have generated much interest in the ...

Anthropogenic and biogenic gas emissions contribute to the formation of secondary organic aerosol (SOA). When present, soot particles from fossil fuel combustion can acquire a coating of SOA. We investigate SOA-soot biogenic-anthropogenic interactions and their impact on ice nucleation in relation to the particles' organic phase state. SOA particles were generated from the OH oxidation of napht...