نتایج جستجو برای: asymmetric catalysis

تعداد نتایج: 90956  

Journal: :DEStech Transactions on Computer Science and Engineering 2017

2017
Yin Zhang Jun Guo Lin Shi Yanfei Zhu Ke Hou Yonglong Zheng Zhiyong Tang

A simple and effective strategy is developed to realize visible light-driven heterogeneous asymmetric catalysis. A chiral organic molecule, which only has very weak catalytic activity in asymmetric α-alkylation of aldehydes under visible light, is utilized as the ligand to coordinate with different types of metal ions, including Zn2+, Zr4+, and Ti4+, for construction of crystalline metal organi...

Journal: :Journal of the American Chemical Society 2013
Elad Gross Jack H Liu Selim Alayoglu Matthew A Marcus Sirine C Fakra F Dean Toste Gabor A Somorjai

Research to develop highly versatile, chiral, heterogeneous catalysts for asymmetric organic transformations, without quenching the catalytic reactivity, has met with limited success. While chiral supramolecular structures, connected by weak bonds, are highly active for homogeneous asymmetric catalysis, their application in heterogeneous catalysis is rare. In this work, asymmetric catalyst was ...

Journal: :Organic & biomolecular chemistry 2015
K G M Kou V M Dong

Sulfoxides are uncommon substrates for transition-metal catalysis due to their propensity to inhibit catalyst turnover. In a collaborative effort with Ken Houk, we developed the first dynamic kinetic resolution (DKR) of allylic sulfoxides using asymmetric rhodium-catalyzed hydrogenation. A detailed mechanistic analysis of this transformation using both experimental and theoretical methods revea...

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