The time-window for processing electron spin information (spintronics) in solid-state quantum electronic devices is determined by the spin-lattice and spin-spin relaxation times of electrons. Minimizing the effects of spin-orbit coupling and the local magnetic contributions of neighbouring atoms on spin-lattice and spin-spin relaxation times at room temperature remain substantial challenges to ...

The electron spin relaxation times measured in ESR spectroscopy are physically distinct from the electron spin relaxation times which appear in the theory of NMR Paramagnetic Relaxation Enhancement ~NMR-PRE!. ESR involves decay of a perturbed spin density matrix toward thermal equilibrium, while in NMR-PRE measurements, the electron spin density matrix remains at thermal equilibrium throughout ...

the molecular weight distribution of 4 commercial isotactic polypropylene (ipp) samples was estimated using rheological data. the dynamic moduli data, obtained from rheological measurements in linear viscoelastic region was used for calculation of relaxation time spectrum, h(τ) and then shear relaxation modulus, g(t). finally, applying thimm kernel function and relaxation modulus data in genera...

Electron-nuclear relaxation dynamics are studied in Hgn 2 (11<n<16,n518) using time-resolved photoelectron imaging. The excess electron in the anion uniquely occupies the p band and is excited intraband by 1.53 eV pump photons; the subsequent dynamics are monitored by photodetachment at 3.06 eV and measurement of the photoelectron images as a function of pump-probe delay. The initially excited ...

Ultrafast, subfemtosecond charge migration in small peptides is discussed on the basis of computational studies and compared with the selective bond dissociation after ionization as observed by Schlag and Weinkauf. The reported relaxation could be probed in real time if the removal of an electron could be achieved on the attosecond time scale. Then the mean field seen by an electron would be ch...

— We have applied the SEDM technique to study the electron hopping time at the octahedral (B) sites in magnetite. We have found that this relaxation time is either zero or less than 10" s at room temperature and 125 K. At 112 K the SEDM results for the octahedral (B) sites are quite different from those at room temperature and 125 K. Relaxation may be occurring, but in the absence of a theoreti...

We have performed mixed quantum-classical molecular dynamics simulations of the relaxation of a ground state excess electron at interfaces of different phases of water with air. The investigated systems included ambient water/air, supercooled water/air, Ih ice/air, and amorphous solid water/air interfaces. The present work explores the possible connections of the examined interfacial systems to...

The electron and hole relaxation in the (7, 0) zigzag carbon nanotube is simulated in time domain using a surface-hopping Kohn-Sham density functional theory. Following a photoexcitation between the second van Hove singularities, the electrons and holes decay to the Fermi level on characteristic subpicosecond time scales. Surprisingly, despite a lower density of states, the electrons relax fast...

The electron spin dynamics in (111)-oriented GaAs/AlGaAs quantum wells is studied by time-resolved photoluminescence spectroscopy. By applying an external electric field of 50 kV/cm a two-order of magnitude increase of the spin relaxation time can be observed reaching values larger than 30 ns; this is a consequence of the electric field tuning of the spin-orbit conduction band splitting which c...

We study the relaxation of a non-equilibrium carrier distribution under the influence of the electron-electron interaction in the presence of disorder. Based on the Anderson model, our Hamiltonian is composed from a single particle part including the disorder and a two-particle part accounting for the Coulomb interaction. We apply the equation-of-motion approach for the density matrix, which pr...