Herein, we demonstrate the ability to optically tune mobility of electrically powered Janus particles (JPs) that are half-coated with various zinc oxide ($\mathrm{Zn}\mathrm{O}$) semiconducting layers, i.e., polycrystalline, amorphous, and amorphous a ${\mathrm{Si}\mathrm{O}}_{2}$ passivation layer. The $\mathrm{Zn}\mathrm{O}$ semiconductor photoresponse causes an increase in its electrical con...