نتایج جستجو برای: nucleophilic substitution reactions

تعداد نتایج: 222918  

Journal: :Physical chemistry chemical physics : PCCP 2012
Nicolas Chéron Denis Jacquemin Paul Fleurat-Lessard

Depending on the selected DFT functional, two different mechanisms are found for two organic reactions (an intramolecular nucleophilic aromatic substitution and a nucleophilic addition on a carbonyl moiety). Indeed, B3LYP predicts a concerted mechanism whereas M06-2X foresees a multistep one. Calculations at the MP4(SDQ) level proved the mechanisms to be stepwise. We studied these reactions wit...

Journal: :Chemical communications 2014
Qian Zhang Xu Liu Xiaoqing Xin Rui Zhang Yongjiu Liang Dewen Dong

A facile and efficient one-pot synthesis of polysubstituted pyridin-2(1H)-ones from readily available enaminones and the cyanomethyl sulfonium bromide salt in the presence of cesium carbonate is developed, and a mechanism involving sequential nucleophilic vinylic substitution (S(N)V), intramolecular nucleophilic cyclization and dealkylation reactions is proposed.

2017
Jiho Song Hae Ju Kang Jung Wuk Lee Michelle A Wenas Seung Hwarn Jeong Taeho Lee Kyungsoo Oh Kyung Hoon Min

In view of the few reports concerning aromatic nucleophilic substitution reactions featuring an alkoxy group as a leaving group, the aromatic nucleophilic substitution of 2,4-dimethoxynitrobenzene was investigated with a bulky t-butoxide nucleophile under microwave irradiation. The transetherification of 2,4-dimethoxynitrobenezene with sodium t-butoxide under specific conditions, namely for 20 ...

Journal: :Chem 2021

The development of new reactions is important to improve the toolbox organic chemistry. One way nudge a reaction undergo pathway different from what it normally takes. Stereoinvertive SN2 known be intolerant bulky tertiary carbon centers, which tend proceed through SN1 pathways form racemized products. This leads long-standing challenge in synthesis; that is, how prepare enantiopure compounds s...

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