This thesis describes the design and construction of two laser systems to probe the 674nm transition of 88Sr+ ions in a linear Paul trap. The first laser system made use of a molecular transition in Iodine to stabilize the length of a Fabry-Perot cavity for laser locking. After constructing this laser, we measured an unsuitable experimental stability of 10 MHz over 5 minutes. A completely new m...

Laser cooling is theoretically investigated in a cascade three-level scheme, where the excited state of a laser-driven transition is coupled by a second laser to a top, more stable level, as for alkaline-earth-metal atoms. The second laser action modifies the atomic scattering cross section and produces temperatures lower than those reached by Doppler cooling on the lower transition. When multi...

The ASACUSA (Atomic Spectroscopy and Collisions Using Slow Antiprotons) collaboration is currently attempting to observe a laser-induced resonant transition of antiprotonic helium atoms at wavelength of 1154.9 nm. Motivations to observe this transition and a nanosecond near-infrared laser prepared for this work are presented.

Excitation of antiferromagnetic HoFeO3 with a single 80 fs laser pulse triggers a first-order spin-reorientation phase transition. In the ultrafast kinetics of the transition one can distinguish the processes of impulsive excitation of spin precession, nucleation of the new domain and growth of the nuclei. The orientation of the spins in the nuclei is defined by the phase of the laser-induced c...

We discuss the production of ultracold molecules in their electronic ground state by photoassociation employing electronically excited states with ion-pair character and strong spin-orbit interaction. A short photoassociation laser pulse drives a nonresonant three-photon transition for alkali-metal atoms colliding in their lowest triplet state. The excited-state wave packet is transferred to th...

Laser filamentation in gases is often carried out in the laboratory with focusing optics to better stabilize the filament, whereas real-world applications of filaments frequently involve collimated or near-collimated beams. It is well documented that geometrical focusing can alter the properties of laser filaments and, consequently, a transition between a collimated and a strongly focused filam...

The absolute frequency of the In(+) 5s(2) (1)S(0)5s5p (3)P(0) clock transition at 237 nm was measured with an accuracy of 1.8 parts in 10(13). Using a phase-coherent frequency chain, we compared the (1)S(0)(3)P(0) transition with a methane-stabilized HeNe laser at 3.39 microm, which was calibrated against an atomic cesium fountain clock. A frequency gap of 37 THz at the fourth harmonic of the H...

We use the magnetic field distribution of an azimuthally polarized focused laser beam to excite a magnetic dipole transition in Eu^{3+} ions embedded in a Y2O3 nanoparticle. The absence of the electric field at the focus of an azimuthally polarized beam allows us to unambiguously demonstrate that the nanoparticle is excited by the magnetic dipole transition near 527.5 nm. When the laser wavelen...

In Arsenic a pressure-induced solid-solid phase transition from the A7 into the simple cubic structure has been experimentally demonstrated [Beister et al. 1990 Phys. Rev. B 41 5535]. In this paper we present calculations, which predict that this phase transition can also be induced by an ultrashort laser pulse in As under pressure. In addition, calculations for the pressure-induced phase trans...