A research effort was carried out at the Bhabha Atomic Research Centre (BARC), Mumbai, for developing laser-based techniques for enrichment of natural uranium to reactor-grade (2.5% to 3.0% U), with the potential to be economically scalable to industrial production. Three approaches – two molecular, namely CO2 laser-based approach and UF6-based approach, and one atomic, namely Atomic Vapour Las...

The work on molten salts and isotope separation performed over the years at Université Pierre et Marie Curie and at Collège de France is critically reviewed. This research, closely related to A. Klemm’s pioneering contributions, leads among other things to the discovery of the effect now called the ‘Chemla effect’, after the late Professor Marius Chemla. These studies of ionic motions in melts,...

The most important demand in an efficient carbon isotope separation is to keep the cryogenic distillation column parameters at their required set points, despite disturbances or uncertainties. One of the key parameters is the column temperature that has a direct influence on the carbon separation coefficient. The nonlinear model of the separation process considers the top and bottom column temp...

In a heterogeneous electrolyte system of a strongly basic anion exchanger and solutions of NaBF4 or NaClC>4 we established the influence of the nature and concentration of the eluent in chromatographic experiments on chlorine isotope separation. Results show that when the electrolyte concentration is increased the degree of isotope separation decreases. With NaBF4 the separation factor is great...