نتایج جستجو برای: hydrogenation of benzene

تعداد نتایج: 21166979  

Journal: :MATEC web of conferences 2021

Rhodium and rhodium-gold catalysts supported on amorphous aluminosilicates (ASA), titanium dioxide (rutile, TiO 2 ) was prepared in two different ways: absorption colloidal method. The were characterized by an inductively coupled plasma optical emission spectrometer (ICP-OES), transmission electron microscopy (TEM) X-ray diffraction (XRD). activity selectivity of the tested hydrogenation benzen...

Journal: :Chemical communications 2012
Wanfang Li Weizheng Fan Xin Ma Xiaoming Tao Xiaoming Li Xiaomin Xie Zhaoguo Zhang

By modulating the chelating priorities of the different directing groups in 3,5-diketo amides with the assistance from coordinating solvent, highly chemo- and enantioselective hydrogenation of the C3-carbonyls was achieved in the presence of [RuCl(benzene)(S)-SunPhos]Cl in THF.

Journal: :Proceedings of the National Academy of Sciences of the United States of America 2013
Linda A Williams Neng Guo Alessandro Motta Massimiliano Delferro Ignazio L Fragalà Jeffrey T Miller Tobin J Marks

Structural characterization of the catalytically significant sites on solid catalyst surfaces is frequently tenuous because their fraction, among all sites, typically is quite low. Here we report the combined application of solid-state (13)C-cross-polarization magic angle spinning nuclear magnetic resonance ((13)C-CPMAS-NMR) spectroscopy, density functional theory (DFT), and Zr X-ray absorption...

2016
Raffaello Papadakis Hu Li Joakim Bergman Anna Lundstedt Kjell Jorner Rabia Ayub Soumyajyoti Haldar Burkhard O Jahn Aleksandra Denisova Burkhard Zietz Roland Lindh Biplab Sanyal Helena Grennberg Klaus Leifer Henrik Ottosson

The first hydrogenation step of benzene, which is endergonic in the electronic ground state (S0), becomes exergonic in the first triplet state (T1). This is in line with Baird's rule, which tells that benzene is antiaromatic and destabilized in its T1 state and also in its first singlet excited state (S1), opposite to S0, where it is aromatic and remarkably unreactive. Here we utilized this fea...

Journal: :Journal of Synthetic Organic Chemistry, Japan 1972

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