نتایج جستجو برای: condensed phase

تعداد نتایج: 610943  

Journal: :Accounts of chemical research 2006
Gabriel Hanna Raymond Kapral

The study of quantum rate processes occurring in condensed phase environments is difficult because of the large number of degrees of freedom involved. Since a full quantum mechanical treatment is not computationally feasible, one is motivated to use mixed quantum-classical dynamical methods. This type of dynamics is applicable when one can single out a few degrees of freedom to be quantum in na...

Journal: :Physical review letters 2008
Xiangyun Qiu Kurt Andresen Jessica S Lamb Lisa W Kwok Lois Pollack

We have investigated the energetics of DNA condensation by multivalent polyamine cations. Solution small angle x-ray scattering was used to monitor interactions between short 25 base pair dsDNA strands in the free supernatant DNA phase that coexists with the condensed DNA phase. Interestingly, when tetravalent spermine is used, significant inter-DNA repulsion is observed in the free phase, in c...

Journal: :The Journal of chemical physics 2004
H J Bakker

A modified Landau-Teller equation for vibrational relaxation in the condensed phase is proposed. This equation differs from previous approaches by accounting for the fluctuations of the energies of the vibrational levels that result from the interactions with the surroundings (bath). In the conventional approach the effects of the bath are only included in the coupling between the relaxing and ...

Journal: :Journal of Chemical Theory and Computation 2014

Journal: :Journal of Physics: Conference Series 2014

2004
P. J. Popp R. S. Gao T. P. Marcy D. W. Fahey P. K. Hudson T. L. Thompson B. Kärcher B. A. Ridley A. J. Weinheimer D. J. Knapp D. D. Montzka D. Baumgardner T. J. Garrett E. M. Weinstock J. B. Smith D. S. Sayres J. V. Pittman S. Dhaniyala T. P. Bui M. J. Mahoney

[1] The redistribution of HNO3 via uptake and sedimentation by cirrus cloud particles is considered an important term in the upper tropospheric budget of reactive nitrogen. Numerous cirrus cloud encounters by the NASA WB-57F high-altitude research aircraft during the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE) were accompanied by the ...

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