We study the optical dynamics in complexes of aluminum nanoantennas coated with molecular J-aggregates and find that they provide an excellent platform for the formation of hybrid exciton-localized surface plasmons. Giant Rabi splitting of 0.4 eV, which corresponds to ∼10 fs energy transfer cycle, is observed in spectral transmittance. We show that the nanoantennas can be used to manipulate the...

Optoelectronic-compatible heterostructures are fabricated from layered inorganic-organic multiple quantum wells (IO-MQW) of Cyclohexenyl ethyl ammonium lead iodide, (C(6)H(9)C(2)H(4)NH(3))(2)PbI(4) (CHPI). These hybrids possess strongly-resonant optical features, are thermally stable and compatible with hybrid photonics assembly. Room-temperature strong-coupling is observed when these hybrids a...

Photon splitting due to vacuum polarization in the electric field of an atom is considered. We survey different theoretical approaches to the description of this nonlinear QED process and several attempts of its experimental observation. We present the results of the lowest-order perturbation theory as well as those obtained within the quasiclassical approximation being exact in the external fi...

Semiconductor-microcavity polaritons are composite quasiparticles of excitons and photons, emerging in the strong coupling regime. As quantum superpositions of matter and light, polaritons have much stronger interparticle interactions compared with photons, enabling rapid equilibration and Bose-Einstein condensation (BEC). Current realizations based on 1D photonic structures, such as Fabry-Péro...

In this theoretical work, we report on voltage-controllable hybridization of electromagnetic modes arising from strong interaction between graphene surface plasmons and molecular vibrations. The interaction strength depends strongly on the volume density of molecular dipoles, the molecular relaxation time, and the molecular layer thickness. Graphene offers much tighter plasmonic field confineme...

We present a quantum model of two-level atoms localized in a three-dimensional lattice based on the Hopfield polariton theory. In addition to a polaritonic gap at the excitation energy, a photonic band gap opens up at the Brillouin zone boundary. Upon tuning the lattice period or angle of incidence to match the photonic gap with the excitation energy, one obtains a combined polaritonic and phot...

We investigate the thermodynamics and signatures of a polariton condensate over a range of densities, using a model of microcavity polaritons with internal structure. We determine a phase diagram for this system including fluctuation corrections to the mean-field theory. At low densities the condensation temperature Tc behaves like that for point bosons. At higher densities, when Tc approaches ...

Wide bandgap semiconductors are attractive candidates for polariton-based devices operating at room temperature. We present numerical simulations of reflectivity, transmission and absorption spectra of bulk GaAs, GaN and ZnO microcavities, in order to compare the particularities of the strong coupling regime in each system. Indeed the intrinsic properties of the excitons in these materials resu...

Hybridized decaying oscillations in a nanosystem of two coupled elements—a quantum emitter and a plasmonic nanoantenna—are considered as a classical effect. The circuit model of the nanosystem extends beyond the assumption of inductive or elastic coupling and implies the near-field dipole-dipole interaction. Its results fit those of the previously developed classical model of Rabi splitting, ho...