Understanding the electronic properties of quasicrystals, in particular the dependence of these properties on dimension, is among the interesting open problems in the field of quasicrystals. We investigate an off-diagonal tight-binding hamiltonian on the separable square and cubic Fibonacci quasicrystals. We use the well-studied singular-continuous energy spectrum of the 1-dimensional Fibonacci...

We report the anion photoelectron spectrum of I2- taken at 5.826 eV detachment energy using velocity mapped imaging. The photoelectron spectrum exhibits bands resulting from transitions to the bound regions of the X 1Sigmag+(0g+), A' 3Piu(2u), A 3Piu(1u), and B 3Piu(0u+) electronic states as well as bands resulting from transitions to the repulsive regions of several I2 electronic states: the B...

Although the mechanism of superconductivity in the cuprates remains elusive, it is generally agreed that at the heart of the problem is the physics of doped Mott insulators. A crucial step for solving the high temperature superconductivity puzzle is to elucidate the electronic structure of the parent compound and the behaviour of doped charge carriers. Here we use scanning tunnelling microscopy...

In this work, we demonstrate the feasibility to collect off-electronic resonance chiral sum frequency generation (SFG) vibrational spectra from interfacial proteins and peptides at the solid/liquid interface in situ. It is difficult to directly detect a chiral SFG vibrational spectrum from interfacial fibrinogen molecules. By adopting an interference enhancement method, such a chiral SFG vibrat...

The dynamics of pyrrole excited at wavelengths in the range 242-217 nm are studied using a combination of time-resolved photoelectron spectroscopy and wavepacket propagations performed using the multi-configurational time-dependent Hartree method. Excitation close to the origin of pyrrole's electronic spectrum, at 242 and 236 nm, is found to result in an ultrafast decay of the system from the i...

Charge carriers in bilayer graphene are widely believed to be massive Dirac fermions that have a bandgap tunable by a transverse electric field. However, a full transport gap, despite its importance for device applications, has not been clearly observed in gated bilayer graphene, a long-standing puzzle. Moreover, the low-energy electronic structure of bilayer graphene is widely held to be unsta...

The Open University's repository of research publications and other research outputs Electronic state spectroscopy of methyl formate probed by high resolution VUV photoabsorption, He(I) photoelectron spectroscopy and ab initio calculations Journal Article (2010). Electronic state spectroscopy of methyl formate probed by high resolution VUV photoabsorption, He(I) photoelectron spectroscopy and a...

The electronic and vibrational absorption spectra of the radical anion and cation of p-benzoquinone (PBQ) in an Ar matrix between 500 and 40,000 cm(-1) are presented and discussed in detail. Of particular interest is the radical cation, which shows very unusual spectroscopic features that can be understood in terms of vibronic coupling between the ground and a very low-lying excited state. The ...

Modern land commanders are increasingly dependent on information-age systems comprising communications and information systems, networks and sensors. While these systems have the potential to produce significant changes in the conduct and character of war, their reliance on the electromagnetic spectrum also has the potential to increase their vulnerability to interdiction by electronic-warfare ...