نتایج جستجو برای: dicationic 4

تعداد نتایج: 1303925  

2012
Heikki Rinta Anssi Peuronen Manu Lahtinen

The asymmetric unit of the title three-dimensional coordination polymer, [Mn2Br6(C11H28N2O2)] n , consists of one Mn(II) cation, half of a dicationic N,N'-bis-(2-hy-droxy-eth-yl)-N,N,N',N'-tetra-methyl-propane-1,3-diaminium ligand (L) (the other half being generated by a twofold rotation axis), and three bromide ions. The Mn(II) cation is coordinated by a single L ligand via the hy-droxy O atom...

An atom-efficient, eco-friendly, solvent-free, high yielding, multicomponent green strategy to synthesize triazolo[1,2-a]indazole-triones derivatives by the one-pot condensation of aldehyde, dimedone, and phenyl urazole is presented. A series of different substituted aromatic aldehydes including either electron-withdrawing or electron-donating groups used in this reaction participated well and ...

The present study, for the first time, presents a feasible protocol for the preparation of β-cyclodextrin/ imidazolium based dicationic ionic liquid, [βCD/Im](OTs)2, and its application as an efficient and eco-friendly microvessel and host ionic liquid system for the regioselective ring opening of the epoxides in water. No evidence for the formation of diol by-products or side reacti...

Journal: :ACS chemical biology 2013
Aaron Bender Zachary R Woydziak Liqiang Fu Michael Branden Zhenguo Zhou Brian D Ackley Blake R Peterson

Unlike the digestive systems of vertebrate animals, the lumen of the alimentary canal of Caenorhabditis elegans is unsegmented and weakly acidic (pH ~4.4), with ultradian fluctuations to pH > 6 every 45-50 s. To probe the dynamics of this acidity, we synthesized novel acid-activated fluorophores termed Kansas Reds. These dicationic derivatives of rhodamine B become concentrated in the lumen of ...

Journal: :Proceedings of the National Academy of Sciences of the United States of America 1996
J E Coury L McFail-Isom L D Williams L A Bottomley

Determining the mode-of-binding of a DNA ligand is not always straightforward. Here, we establish a scanning force microscopic assay for mode-of-binding that is (i) direct: lengths of individual DNA-ligand complexes are directly measured; (ii) rapid: there are no requirements for staining or elaborate sample preparation; and (iii) unambiguous: an observed increase in DNA length upon addition of...

2017
D. You H. Fukuzawa Y. Sakakibara T. Takanashi Y. Ito G. G. Maliyar K. Motomura K. Nagaya T. Nishiyama K. Asa Y. Sato N. Saito M. Oura M. Schöffler G. Kastirke U. Hergenhahn V. Stumpf K. Gokhberg A. I. Kuleff L. S. Cederbaum K Ueda

Inner-shell ionization of an isolated atom typically leads to Auger decay. In an environment, for example, a liquid or a van der Waals bonded system, this process will be modified, and becomes part of a complex cascade of relaxation steps. Understanding these steps is important, as they determine the production of slow electrons and singly charged radicals, the most abundant products in radiati...

2001
Krzysztof Bielawski Anna Bielawska

The DNA binding properties of three novel extended aromatic bisamidines (1–3) possessing different dicationic terminal side chains were studied. Data from the ethidium displacement assay showed that bisamidines 1–3 have significant affinity for DNA. We studied the cytotoxic activity of bisamidines 1–3 and Hoechst 33258 in the cultured breast cancer MCF-7 cells. These data show that in broad ter...

2010
Volker Ulrich Silko Barth Toralf Lischke Sanjeev Joshi Tiberiu Arion Melanie Mucke Marko Förstel Alex M. Bradshaw Uwe Hergenhahn Kai Siegbahn

Photoelectron-Auger electron coincidence spectroscopy probes the dicationic states produced by Auger decay following the photoionization of core or inner valence levels in atoms, molecules or clusters. Moreover, the technique provides valuable insight into the dynamics of core hole decay. This paper serves the dual purpose of demonstrating the additional information obtained by this technique c...

2012
Tingting Lu Ming Lu Wang Yu Zhongjie Liu

PEG 1000–based functional dicationic acidic ionic liquid (PEG1000 –DAIL) was used for the first time as the reaction solvent for the N-Hydroxyphthalimide (NHPI)-cobalt acetate(Co(OAc)2) catalyzed aerobic oxidations of alkylaromatics to the corresponding acids. It enhanced the efficient catalytic ability of NHPI: 99.9 % conversion of toluene with 99.5 % selectivity for benzoic acid could be obta...

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