نتایج جستجو برای: cuii determination

تعداد نتایج: 251442  

2016
María José Heras Ojea Victoria A Milway Gunasekaran Velmurugan Lynne H Thomas Simon J Coles Claire Wilson Wolfgang Wernsdorfer Gopalan Rajaraman Mark Murrie

We report a series of 3d-4f complexes {Ln2 Cu3 (H3 L)2 Xn } (X=OAc(-) , Ln=Gd, Tb or X=NO3 (-) , Ln=Gd, Tb, Dy, Ho, Er) using the 2,2'-(propane-1,3-diyldiimino)bis[2-(hydroxylmethyl)propane-1,3-diol] (H6 L) pro-ligand. All complexes, except that in which Ln=Gd, show slow magnetic relaxation in zero applied dc field. A remarkable improvement of the energy barrier to reorientation of the magnetis...

Journal: :Applied Physics Letters 2021

Jahn–Teller distortions are often observed in CuII-containing complex oxides resulting remarkable changes of physical properties. Tuning the with pressure has attracted considerable interest but is less studied high-entropy (HEOs). We found that can suppress structural originating from effect CuO6 octahedra rock salt-type (Mg0.2Ni0.2Co0.2Zn0.2Cu0.2)O HEO and significantly modify its electronic ...

Journal: :Dalton transactions 2015
Pedro Adão Sónia Barroso M Fernanda N N Carvalho Carlos M Teixeira Maxim L Kuznetsov João Costa Pessoa

We report the synthesis and characterization of several novel aminopyridine - L-amino acid derived Cu(II)-complexes. The ligands are prepared by a one-pot reductive alkylation of the L-amino acid scaffold and the respective aminopyridine Cu(II)-complexes were obtained by reaction with CuCl2 or Cu(acetato)2. All compounds were characterized by spectroscopic techniques, as well as ESI-MS. Two of ...

Journal: :Chemical communications 2006
Thorsten Glaser Ioannis Liratzis Olga Kataeva Roland Fröhlich Manuel Piacenza Stefan Grimme

Two hydrogen-bonds from geometrically constrained OH groups to coordinated oxygen donors shift the reduction potential of a Cu(II) complex by +270 mV as compared to the structurally analogous reference complex missing the OH groups.

Journal: :Angewandte Chemie 2021

Metal-catalyzed C–N cross-coupling generally forms C−N bonds by reductive elimination from metal complexes bearing covalent C- and N-ligands. We have identified a Cu-mediated that uses dative N-ligand in the bond-forming event, which, contrast to conventional methods, generates reactive cationic products. Mechanistic studies suggest process operates via transmetalation of an aryl organoboron Cu...

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