Comparisons with respect to the sooting tendency are made between stationary diffusion flames and diffusion flames with pulsations induced by oscillating fuel flow. Time-resolved measurements of the soot particle properties in the flames are obtained by combining Rayleigh-scattering, laser-induced incandescence, and extinction measurements into the RAYLIX method. Furthermore, flame luminosity a...

[1] During Transport and Chemical Evolution over the Pacific (TRACE-P) and Asian Aerosol Characterization Experiment (ACE-Asia) we measured the dry size distribution of Asian aerosols, their state of mixing, and the optical properties of dust, black carbon (BC) and other aerosol constituents in combustion and/or dust plumes. Optical particle sizing in association with thermal heating extracted ...

[1] This study examines the short‐term (∼15 year) effects of controlling fossil‐fuel soot (FS) (black carbon (BC), primary organic matter (POM), and S(IV) (H2SO4(aq), HSO4 , and SO4 )), solid‐biofuel soot and gases (BSG) (BC, POM, S(IV), K, Na, Ca, Mg, NH4 , NO3 , Cl and several dozen gases, including CO2 and CH4), and methane on global and Arctic temperatures, cloudiness, precipitation, and at...

The impact of organic carbon (OC) on the light absorption soot is determined by discrete element modeling coupled with dipole approximation for computing scattering radiation particles. mass cross-section (MAC) used widely to determine its absorption. Typically MAC obtained from average refractive index OC and elemental (EC) large C/H that make up mature soot. As such, can be overestimated a fa...

AS MORPHOLOGY PLAYS A RELEVANT ROLE IN SOLID/SOLID CATALYSIS, WHERE THE NUMBER OF CONTACT POINTS IS A CRITICAL FEATURE IN THIS KIND OF REACTION, THREE DIFFERENT CERIA MORPHOLOGIES HAVE BEEN INVESTIGATED IN THIS WORK AS SOOT OXIDATION CATALYSTS: ceria nanofibers, which can become organized as a catalytic network inside diesel particulate filter channels and thus trap soot particles at several co...

The emission of solid carbonaceous particulate matter (i.e. soot) is a world-wide problem that effects both human health and global environmental health alike. Although a number of sources contribute to the concentration of soot in the atmosphere, Diesel engines play a significant role. Diesel engines, or direct-injection compression-ignition engines, are the primary power plant for delivering ...

We present a detailed set of measurements from a piloted, sooting, turbulent C2H4fueled diffusion flame. Hybrid femtosecond/picosecond coherent anti-Stokes Raman scattering (CARS) is used to monitor temperature and oxygen, while laser-induced incandescence (LII) is applied for imaging of the soot volume fraction in the challenging jet-flame environment at Reynolds number, Re = 20,000. Single-la...

In this article we present a parameter free aggregation model for soot formation. Each soot particle is represented as a fractal aggregate that can be described by its total volume, total surface, and number of hydrogenated sites on its surface. The moments of the joint Probility Density Function (PDF) of these three quantities are solved using the Direct Quadrature Method of Moments (DQMOM). T...

A novel method for soot detection based on SiC MOSFET devices with a dual suspended/ floating gate configuration in a co-fired LTCC package has been investigated. Response to different concentrations of soot was measured through the application of an electric field between the two gate electrodes to attract charged soot onto the sensor surface. Results are promising with ap plication areas from...