Abstract. High-mercury wet deposition in the southeastern United States has been noticed for many years. Previous studies came up with a theory that it was associated high-altitude divalent mercury scavenged by convective precipitation. Given coarse resolution of previous models (e.g., GEOS-Chem), this is still not fully tested. Here we employed newly developed WRF-GEOS-Chem (WRF-GC; WRF: Weath...

WRF-Chem simulations of aerosol seasonal variability in the San Joaquin Valley (SJV), California, are evaluated by satellite and in situ observations. Results show that the WRF-Chem model successfully captures the distribution and magnitude of and variation in SJV aerosols during the cold season. However, aerosols are not well represented in the warm season. Aerosol simulations in urban areas d...

A Real-Time Air Quality Forecast (RT-AQF) system that is based on a three-dimensional air quality model provides a powerful tool to forecast air quality and advise the public with proper preventive actions. In this work, a new RT-AQF system is developed based on the online-coupled Weather Research and Forecasting model with Chemistry (WRF/Chem) with the Model of Aerosol Dynamics, Reaction, Ioni...

We have applied the MM5-CMAQ model to simulate the high concentrations in PM10 and PM2.5 during a winter episode (2003) in Central Europe. The selected period is January 15 – April 6 2003. Values of daily mean concentrations up to 75 μgm are found on average of several monitoring stations in Northern Germany. This model evaluation shows that there is an increasing underestimation of primary and...

We have made a number of developments to the Weather, Research and Forecasting model coupled with Chemistry (WRF-Chem), with the aim of improving model prediction of trace atmospheric gas-phase chemical and aerosol composition, and of interactions between air quality and weather. A reduced form of the Common Reactive Intermediates gas-phase chemical mechanism (CRIv2-R5) has been added, using th...