All-solid-state batteries with inorganic solid electrolytes (SEs) are recognized as an ultimate goal of rechargeable batteries because of their high safety, versatile geometry, and good cycle life. Compared with thin-film batteries, increasing the reversible capacity of bulk-type all-solid-state batteries using electrode active material particles is difficult because contact areas at solid–soli...

All-solid-state sodium-ion batteries are promising candidates for large-scale energy storage applications. The key enabler for an all-solid-state architecture is a sodium solid electrolyte that exhibits high Na(+) conductivity at ambient temperatures, as well as excellent phase and electrochemical stability. In this work, we present a first-principles-guided discovery and synthesis of a novel C...

Lithium ion secondary batteries have a high voltage and a high energy density, as shown in Fig. 1, and are widely used in mobile devices such as cell phones, notebook PCs and PDAs. However, since lithium ion secondary batteries use a flammable organic liquid electrolyte, there is a risk of explosion or fire. Fire accidents can also occur due to contamination during production or from overchargi...

A unique way of robustly integrating an elastomer fi lm onto a graphitic anode and then post-process it into a solid-state electrolyte for lithium-ion battery applications is reported. The mutual solvability of the elastomer and the binder of the graphitic anode (carboxymethyl cellulose, (CMC)) in dimethylformamide facilitates the fusion of the two heterogeneous layers. Dimensional dynamics evo...

All-solid-state Li-ion batteries based on ceramic solid electrolyte materials are a promising next-generation energy storage technology with high energy density and enhanced cycle life. The poor interfacial conductance is one of the key limitations in enabling all-solid-state Li-ion batteries. However, the origin of this poor conductance has not been understood, and there is limited knowledge a...

All-solid-state lithium-ion batteries using Li+-ion conducting ceramic electrolytes have been focused on as attractive future batteries for electric vehicles and renewable energy conversion systems because high safety can be realized due to non-flammability of ceramic electrolytes. In addition, a higher volumetric energy density than that of current lithium-ion batteries is expected since the a...

The supply and the management of the energy are particularly at the centre of our daily concerns and represent a socio-economic priority. Indeed, while cars use fossil fuel as the main source of energy for over a century, the depletion of the oil reserves and the necessity to reduce the carbon dioxide emissions, stimulate the development of electric vehicles. Therefore, one of the main challeng...