In a series of simulations with the global ECHAM5-HAM aerosol-climate model, the response to changes in anthropogenic emissions is analyzed. Traditionally, additivity is assumed in the assessment of the aerosol climate impact, as the underlying bulk aerosol models are largely constrained to linearity. The microphysical aerosol module HAM establishes degrees of freedom for nonlinear responses of...

[1] Aircraft observations of carbon monoxide (CO) from the ICARTT campaign over the eastern United States in summer 2004 (July 1–August 15), interpreted with a global 3-D model of tropospheric chemistry (GEOS-Chem), show that the national anthropogenic emission inventory from the U.S. Environmental Protection Agency (93 Tg CO y ) is too high by 60% in summer. Our best estimate of the CO anthrop...

A series of analyses were performed to provide chemical signatures for surface soils and to evaluate potential sources of fugitive dust in the Paso del Norte (PdN) region. Eighteen sites were selected for soil sampling based on an assessment of the soil types in the region and the main upwind source areas with a potential for wind erosion. Analyses of the soil samples provided chemical 'fingerp...

This study provides a new approach to estimate both anthropogenic non-point-source and point-source nitrogen (N) inputs to the landscape, and determines their impacts on riverine ammonia–nitrogen (AN) flux, providing a foundation for further exploration of anthropogenic effects on N pollution. Our study site is Huai River basin of China, a watershed with one of the highest levels of N input in ...

A Lagrangian approach based on a physical-biogeochemical modeling was used to compare the potential transfer of cadmium (Cd) from natural and anthropogenic sources to plankton communities (Cd-uptake) in the North-West African upwelling. In this region, coastal upwelling was estimated to be the main natural source of Cd while the most significant anthropogenic source for marine ecosystem is prov...

Platinum, palladium, rhodium, iridium and osmium were found to be enriched relative to their expected natural concentrations in peat samples from Thoreau's Bog, an ombrotrophic peat bog in Concord, Massachusetts. The source of osmium into the bog was determined from its isotopic composition (187Os/188Os). Osmium is composed of 4% lithogenic osmium from atmospheric soil dust, 41% of anthropogeni...

We examine the trans-Pacific transport of mercury using a global chemical transport model. Using existing anthropogenic inventories, the model reproduces the observed Hg/CO ratio in Asian long-range transport events observed at a surface site in Okinawa, Japan and Mount Bachelor, Oregon, with an underestimate of 18-26% in the ratio. This is in contrast with previous studies that inferred a fact...

Global models estimate that the anthropogenic component of atmospheric nitrogen (N) deposition to the ocean accounts for up to a third of the ocean's external N supply and 10% of anthropogenic CO2 uptake. However, there are few observational constraints from the marine atmospheric environment to validate these findings. Due to the paucity of atmospheric organic N data, the largest uncertainties...

heavy metal contamination around the national iranian lead and zinc company (nilz) in zanjan province was evaluated in this paper. collected data were used to appraise the degree of soil contamination and also the source of pollution in the study area based on geoaccumulation index (igeo), and enrichment factor (ef). the levels of fe, zn, cd and pb in the samples exceed those reported in litera...