نتایج جستجو برای: amino alcohols

تعداد نتایج: 217020  

Journal: :Organic letters 2003
Naidu S Chowdari D B Ramachary Carlos F Barbas

[reaction: see text] l-Proline catalyzed the enzyme-like direct asymmetric assembly of aldehydes, ketones, and azodicarboxylic acid esters to provide optically active beta-amino alcohols. This assembly reaction uses both aldehydes and ketones as donors in one pot. The aldol-derived stereocenter is formed with a reduced facial selectivity in reactions involving (R)-amino aldehydes. The reactions...

Journal: :Chemical communications 2015
Tomoya Nobuta Guozhi Xiao Diego Ghislieri Kerry Gilmore Peter H Seeberger

Five active pharmaceutical ingredients (APIs) containing the vicinyl amino alcohol moiety were synthesized using a convergent chemical assembly system. The continuous system is composed of four flow reaction modules: biphasic oxidation, Corey-Chaykovsky epoxidation, phenol alkylation, and epoxide aminolysis. Judicious choice of reagents and module order allowed for two classes of β-amino alcoho...

Journal: :Chemical communications 2012
Minkyoung Kim Kondaji Gajulapati Chorong Kim Hwa Young Jung Jail Goo Kyeong Lee Navneet Kaur Hyo Jin Kang Sang J Chung Yongseok Choi

A variety of diazepinone derivatives were prepared from α-amino acids and amino alcohols by a new synthetic methodology based on ring closing metathesis as a key step. The diazepinones were coupled with ribose derivatives to afford novel diazepinone nucleosides. Among them, (4R)-1-ribosyl-4-methyl-3,4-dihydro-1H-1,3-diazepin-2(7H)-one (3) showed a potent inhibitory effect (K(i) = 145.97 ± 4.87 ...

Journal: :Chem catalysis 2023

Carbon–carbon (C–C) bonds are challenging to selectively cleave owing their chemical inertness and omnipresence in organic molecules; however, they can be targeted during the late-stage modification of natural products active pharmaceutical ingredients. Herein, we report a selective deconstructive C(sp3)–C(sp3) bond cleavage difunctionalization unactivated alcohols mediated by vanadium visible-...

Journal: :Chemical communications 2015
Ai-Jie Cai Yan Zheng Jun-An Ma

A novel, three-component C-C, C-N and C-O bond forming reaction is described. In the presence of 20 mol% CuO, this condensation reaction of CF3CHN2, nitriles, and aldehydes proceeds to afford CF3-substituted oxazolines in moderate to high yields with excellent diastereoselectivities. Subsequent ring-opening of oxazolines gives rise to the corresponding vicinal amino alcohols.

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