[1] Models of aerosol scavenging and aqueous-phase oxidation of SO2 by H2O2 and O3 in a cloud updraft are compared. Bulk models considering only a single droplet size are compared with size-resolved models that explicitly simulate multiple aerosol and drop sizes. All models simulate growth of cloud drops on a lognormal ammonium bisulfate aerosol distribution, and subsequent aqueous-phase chemis...

Estimation of Direct Climate Forcing (DCF) due to aerosols in cloudy areas has historically been a difficult task, mainly because of a lack of appropriate measurements. Recently, passive remote sensing instruments have been developed that have the potential to retrieve both cloud and aerosol properties using polarimetric, multiple view angle, and multi spectral observations, and therefore deter...

To understand the regional impact of the atmospheric aerosols on the surface energy and water cycle in the southern Sierra Nevada characterized by extreme variations in terrain elevation, the authors examine the aerosol radiative forcing on surface insolation and snowmelt for the spring of 1998 in a regional climate model experiment. With a prescribed aerosol optical thickness of 0.2, it is fou...

The aerosol chemical composition in air masses affected by wildfires from the Greek islands of Chios, Euboea and Andros, the Dalmatian Coast and Sicily, during late summer of 2012 was characterized at the remote background site of Finokalia, Crete. Air masses were transported several hundreds of kilometers, arriving at the measurement station after approximately half a day of transport, mostly ...

Aerosol signatures observed by ceilometers are frequently used to derive mixing-layer height (MLH) which is an essential variable for air quality modelling. However, Doppler wind lidar measurements of vertical velocity can provide a more direct estimation of MLH via simple thresholding. A case study reveals difficulties in the aerosol-based MLH retrieval during transition times when the mixing ...

[1] This series of three papers addresses the representation of secondary organic aerosol (SOA) in atmospheric models. SOA forms when gas-phase organic species undergo oxidation, leading to products of sufficiently low vapor pressure that can partition between the gas and aerosol phases. The present paper, part 1, is devoted to the development of a gas-phase atmospheric chemical mechanism desig...

OCTOBER 2004 AMERICAN METEOROLOGICAL SOCIETY | T he Progressive Aerosol Retrieval and Assimilation Global Observing Network (PARAGON) concept (Diner et al. 2004) envisions a coordinated and systematic approach for dramatically improving our understanding of aerosol climate impacts and environmental interactions. Among its scientific motivations is the need to establish, with great confidence, t...

During four aircraft field experiments with the DLR research aircraft Falcon in 1998 (LACE), 2006 (SAMUM-1) and 2008 (SAMUM-2 and EUCAARI), airborne High Spectral Resolution Lidar (HSRL) and in situ measurements of aerosol microphysical and optical properties were performed. Altogether, the properties of six different aerosol types and aerosol mixtures – Saharan mineral dust, Saharan dust mixtu...

Mass transfer effects in hygroscopic measurements of aerosol particles M. N. Chan and C. K. Chan Environmental Engineering Program, School of Engineering, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong Department of Chemical Engineering, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong Received: 2 May 2005 – Accepted: 12 Ma...