نتایج جستجو برای: tropsch

تعداد نتایج: 1156  

2006
M. Luo

Following WW II, it appeared that there would be a severe shortage of crude oil so that U.S. organizations initiated work on Fischer-Tropsch synthesis (FTS). Over a ten year period, the U.S. Bureau of Mines was budgeted $85 million for work on direct and indirect coal liquefaction. These funds would represent more than a billion dollars in today’s marketplace. A large (75 bbl/day) FTS pilot pla...

2015
Morris D. Argyle

Deactivation of heterogeneous catalysts is a ubiquitous problem that causes loss of catalytic rate with time. This review on deactivation and regeneration of heterogeneous catalysts classifies deactivation by type (chemical, thermal, and mechanical) and by mechanism (poisoning, fouling, thermal degradation, vapor formation, vapor-solid and solid-solid reactions, and attrition/crushing). The key...

Journal: :Journal of the American Chemical Society 2013
Anders Tuxen Sophie Carenco Mahati Chintapalli Cheng-Hao Chuang Carlos Escudero Elzbieta Pach Peng Jiang Ferenc Borondics Brandon Beberwyck A Paul Alivisatos Geoff Thornton Way-Faung Pong Jinghua Guo Ruben Perez Flemming Besenbacher Miquel Salmeron

In situ soft X-ray absorption spectroscopy (XAS) was employed to study the adsorption and dissociation of carbon monoxide molecules on cobalt nanoparticles with sizes ranging from 4 to 15 nm. The majority of CO molecules adsorb molecularly on the surface of the nanoparticles, but some undergo dissociative adsorption, leading to oxide species on the surface of the nanoparticles. We found that th...

Journal: :The journal of physical chemistry letters 2017
Zhangzhang Cui Chenlu Xie Xuefei Feng Nigel Becknell Peidong Yang Yalin Lu Xiaofang Zhai Xiaosong Liu Wanli Yang Yi-De Chuang Jinghua Guo

Cobalt-based catalysts are widely used to produce liquid fuels through the Fischer-Tropsch (FT) reaction. However, the cobalt nanocatalysts can exhibit intriguing size-dependent activity whose origin remains heavily debated. To shed light on this issue, the electronic structures of cobalt nanoparticles with size ranging from 4 to 10 nm are studied using soft X-ray absorption (XAS) and resonant ...

2003
Tanya J. Cordes Curtis J. Czerwinski

Hydroxycarbene complexes have been proposed as intermediates in industrial processes such as the Fischer-Tropsch process and hydroformylation. As part of the overall synthesis of an aryltethered version of a chromium hydroxycarbene complex we have examined three synthetic routes toward the brominated biphenyl chromium tricarbonyl compound (η-2’-bromobiphenyl)Cr(CO)3, which is an immediate precu...

2012
Weixin Qian Haitao Zhang Hongfang Ma Yongdi Liu Weiyong Ying Dingye Fang

The adsorption properties of CO and H2 on iron-based catalyst with addition of Zr and Ni were investigated using temperature programmed desorption process. It was found that on the carburized iron-based catalysts, molecular state and dissociative state CO existed together. The addition of Zr was preferential for the molecular state adsorption of CO on iron-based catalyst and the presence of Ni ...

Journal: :Bioresource technology 2013
Qiangu Yan Fei Yu Jian Liu Jason Street Jinsen Gao Zhiyong Cai Jilei Zhang

A continuous process involving gasification, syngas cleaning, and Fischer-Tropsch (FT) synthesis was developed to efficiently produce synthetic aviation turbine fuels (SATFs). Oak-tree wood chips were first gasified to syngas over a commercial pilot plant downdraft gasifier. The raw wood syngas contains about 47% N(2), 21% CO, 18% H(2), 12% CO(2,) 2% CH(4) and trace amounts of impurities. A pur...

2013
E. Virmond J. D. Rocha R. F. P. M. Moreira

Besides high industrial development, Brazil is also an agribusiness country. Each year about 330 million metrics tons (Mg) of biomass residues are generated, requiring tremendous effort to develop biomass systems in which production, conversion and utilization of bio-based products are carried out efficiently and under environmentally sustainable conditions. For the production of biofuels, orga...

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