We investigate the influence of localized and propagating surface plasmons on third harmonic generation from rectangular apertures in metal films. We designed optimal aperture array structures by using finite-difference time-domain simulations with nonlinear scattering theory. From this design space, we fabricated and measured the third harmonic in the region of maximal performance. We find the...

We theoretically show that coaxial waveguides composed of a metallic core, surrounded by a dielectric cylinder and clad by a metal outer layer exhibit negative refractive index modes over a broad spectral range in the visible. For narrow dielectric gaps (10 nm GaP embedded in Ag) a figure-of-merit of 18 can be achieved at lambda(0) = 460 nm. For larger dielectric gaps the negative index spectra...

We study the optical excitation of high-order surface plasmon resonance modes in individual Ag nanorice particles using dark-field scattering spectroscopy. We analyze the results by model calculations using the boundary element method. Symmetry breaking caused by oblique illumination makes the even order resonance modes observable in the optical spectrum. All the resonance peaks are found to re...

We have studied the evolution of dipole-dipole all-plasmonic Fano resonances (FRs) in symmetric multilayered nanoshells as a function of their geometrical parameters. We demonstrate that symmetry breaking is not mandatory for controlling the Fano resonance in such multilayer structures. By carefully selecting the geometrical parameters, the position of the FR can be tuned between 600 and 950 nm...

A matrix balanced version of the recursive centered T matrix algorithm applicable to systems possessing resonant interparticle couplings is presented. Possible domains of application include systems containing interacting localized plasmon resonances, surface resonances, and photonic jet phenomena. This method is of particular interest when considering modifications to complex systems. The nume...

A periodic array of extruded nanoprisms is proposed to generate surface plasmon resonances for sensing applications. Nanoprisms guide and funnel light towards the metal-dielectric interface where the dielectric acts as the medium under test. The system works under normal incidence conditions and is spectrally interrogated. The performance is better than the classical Kretschmann configurations,...

The propagation of laser-excited surface plasmons along a gold film with surface roughness is directly observed via scattered light. The attenuation length of surface plasmons in a broad wavelength interval is calculated for smooth gold and silver films. The surface roughness, which was characterized with an AFM, introduces corrections to the attenuation length, angular dependence of the surfac...

We report the experimental realization of coherent electron spin flip in a modulation-doped CdTe quantum well. Coherent spin rotation is realized with an off-resonant laser pulse, which induces a polarization-dependent optical Stark shift in the trion resonance. Complete electron spin flip is made possible by a laser pulse designed to avoid excessive excitations of nearby exciton resonances and...

Green synthesis of silver nanoparticles (AgNPs) involves a reduction reaction metal salt solution mixed with plant extract. The yield can be controlled using several independent factors, such as extract and concentration, temperature, incubation time. AgNPs from Origanum vulgare (oregano) were synthesized in the past. However, no investigations performed on combined effects factors that affect ...