To design a multiferroic material at atomic scale, strong spin-lattice and charge-lattice couplings play crucial roles. Our first-principles calculation on (SrCoO3)1/(SrTiO3)1 superlattices, with above coupling properties, yields a rich physical phase diagram as a function of epitaxial strain. In particular, a robust ferroelectric ferromagnetic insulator of Pc symmetry is stabilized at tensile ...