نتایج جستجو برای: quantum yield
تعداد نتایج: 482560 فیلتر نتایج به سال:
We broadly generalise Mermin-type arguments on GHZ states, and we provide exact group-theoretic conditions for non-locality to be achieved. Our results are of interest in quantum foundations, where they yield a new hierarchy of quantum-realisable All-vsNothing arguments. They are also of interest to quantum protocols, where they find immediate application to a non-trivial extension of the hybri...
We derive dissipative effective Hamiltonian for the unstable Lee model without any ad hoc coarse graining procedure. Generalized radiative corrections, utilizing the in-in formalism of quantum field theory, automatically yield irreversibility as well as the decay of quantum coherence. Especially we do not need to extend the ordinary Hilbert space for describing the intrinsically dissipative sys...
We describe quantum-field-theoretical (QFT) techniques for mapping quantum problems onto c-number stochastic problems. This approach yields results which are identical to phase-space techniques [C.W. Gardiner, Quantum Noise (1991)] when the latter result in a Fokker-Planck equation for a corresponding pseudo-probability distribution. If phase-space techniques do not result in a Fokker-Planck eq...
Integrability of the quantum Boussinesq equation for c = −2 is demonstrated by giving a recursive algorithm for generating explicit expressions for the infinite number of commuting charges based on a reduction of the W∞ algebra. These charges exist for all spins s ≥ 2. Likewise, reductions of the W∞/2 and W(1+∞)/2 algebras yield the commuting quantum charges for the quantum KdV equation at c = ...
The mechanisms underlying the wavelength dependence of the quantum yield for CO(2) fixation (α) and its acclimation to the growth-light spectrum are quantitatively addressed, combining in vivo physiological and in vitro molecular methods. Cucumber (Cucumis sativus) was grown under an artificial sunlight spectrum, shade light spectrum, and blue light, and the quantum yield for photosystem I (PSI...
High fluorescence quantum yield graphene quantum dots (GQDs) have showed up as a new generation for bioimaging. In this work, luminescent GQDs were prepared by an ameliorative photo-Fenton reaction and a subsequent hydrothermal process using graphene oxide sheets as the precursor. The as-prepared GQDs were nanomaterials with size ranging from 2.3 to 6.4 nm and emitted intense green luminescence...
Cu(I)-responsive fluorescent probes based on a photoinduced electron transfer (PET) mechanism generally show incomplete fluorescence recovery relative to the intrinsic quantum yield of the fluorescence reporter. Previous studies on probes with an N-aryl thiazacrown Cu(I)-receptor revealed that the recovery is compromised by incomplete Cu(I)-N coordination and resultant ternary complex formation...
In this work, we systematically investigated the plasmonic effect on blinking, photon antibunching behavior and biexciton emission of single CdSe/CdS core/shell quantum dots (QDs) near gold nanoparticles (NPs) with a silica shell (Au@SiO2). In order to obtain a strong interaction between the plasmons and excitons, the Au@SiO2 NPs and CdSe/CdS QDs of appropriate sizes were chosen so that the pla...
This paper describes the use of a phenyl bis(dithiocarbamate) (PBTC) linker to enhance the quantum yield of photoinduced electron transfer (eT) from a zinc porphyrin (ZnP) molecule (donor) to a CdSe quantum dot (QD) (acceptor), where quantum yield is defined as the fraction of photoexcited ZnP molecules in the sample that donate an electron to the QD. The PBTC ligand links the ZnP to the QD by ...
In this work, luminescent CdSe@CdS dot-in-rod nanocrystals, CdSe@CdS/ZnS nanorods as well as CdSe-CdS core-crown nanoplatelets were transferred into aqueous phase via ligand exchange reactions. For this purpose, bifunctional thiol-based ligands were employed, namely mercaptoacetic acid (MAA), 3-mercaptopropionic acid (MPA), 11-mercaptoundecanoic acid (MUA) as well as 2-(dimethylamino)ethanthiol...
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