نتایج جستجو برای: epr ii

تعداد نتایج: 588089  

2016
Lawrence J. Berliner

Since the first EPR/ESR spectrum of a paramagnetic substance was published over 70 years ago, the technical improvements did not occur until after/during World War II with the advent of radar technology. The approaches to biomedical problems started somewhat later with the real burst of activity starting after the birth of the spin label technique about 50 years ago. The applications to protein...

Journal: :The Journal of biological chemistry 1974
G Rotilio L Calabrese B Mondovì W E Blumberg

1. EPR spectra of cobalt-copper bovine superoxide dismutase at liquid nitrogen and liquid helium temperature show that the two metal centers are magnetically coupled. The temperature dependence of the spectra indicates that this coupling arises from an exchange interaction. 2. The EPR spectrum of the Co(I1) of the enzyme can only be seen after reduction of the Cu(II), at very low temperature. I...

Journal: :Proceedings of the National Academy of Sciences of the United States of America 2011
John McCoy Wayne L Hubbell

Identifying equilibrium conformational exchange and characterizing conformational substates is essential for elucidating mechanisms of function in proteins. Site-directed spin labeling has previously been employed to detect conformational changes triggered by some event, but verifying conformational exchange at equilibrium is more challenging. Conformational exchange (microsecond-millisecond) i...

Journal: :journal of physical and theoretical chemistry 0
fatih ucun department of physics, faculty of arts and sciences, süleyman demirel university, 32260 isparta, turkey serkan kaya department of physics, faculty of arts and sciences, süleyman demirel university, 32260 isparta, turkey

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پایان نامه :دانشگاه آزاد اسلامی - دانشگاه آزاد اسلامی واحد تهران مرکزی - دانشکده علوم پایه 1391

در این پژوهش نمونه های نانو ساختار هیدروکسی اپتایت با قرار گرفتن در مجاورت گاز ? co?_2 در زمانهای 30و120 و 360 دقیقه تحت درجه حرارت c ° 400 و c ° 100 کربناته شدند. تشکیل کربن اپتایت به روش قرار دادن نمونه ها تحت نفوذ گاز ? co?_2 ، توسط آزمونهای xrd tem ,ftir مورد تائید قرار گرفت. سپس نمونه ها تحت تابش چشمه 60co ?-ray قرارگرفتند و شدت سیگنال epr آنها در دزهای 2, 5, 10, 20, 50و 80 kgy اندازه گرفت...

Journal: :Chemical communications 2015
Yi-Fei Deng Tian Han Zhenxing Wang Zhongwen Ouyang Bing Yin Zhiping Zheng J Krzystek Yan-Zhen Zheng

Two mononuclear square-planar Cr(II) complexes are reported, exhibiting field-induced slow magnetic relaxation. The axial zero-field splitting parameter was unambiguously determined by both a high-frequency/field electron paramagnetic resonance (HF-EPR) technique and magnetic measurements. This result represents the first observed single-molecule-magnet behavior in the square planar coordinatio...

Journal: :Biochimica et Biophysica Acta (BBA) - Bioenergetics 1995

Journal: :Chemical communications 2015
C Lichtenberg L Viciu M Vogt R E Rodríguez-Lugo M Adelhardt J Sutter M M Khusniyarov K Meyer B de Bruin E Bill H Grützmacher

A low-valent trinuclear iron complex with an unusual linear Fe(I)-Fe(II)-Fe(I) unit is presented. It is accessed in a rational approach using a salt metathesis reaction between a new anionic Fe(I) containing heterocycle and FeCl2. Its electronic structure was studied by single crystal XRD analysis, EPR and Mössbauer spectroscopy, and magnetic susceptibility measurements.

Journal: :Chemical communications 2014
Olga V Makhlynets Williamson N Oloo Yurii S Moroz Irina G Belaya Taryn D Palluccio Alexander S Filatov Peter Müller Matthew A Cranswick Lawrence Que Elena V Rybak-Akimova

Mechanistic studies of H2O2 activation by complexes related to [(BPMEN)Fe(II)(CH3CN)2](2+) with electron-rich pyridines revealed that a new intermediate formed in the presence of acetic acid with a 465 nm visible band can be associated with an unusual g = 2.7 EPR signal. We postulate that this chromophore is an acylperoxoiron(III) intermediate.

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