We consider the interaction of quantum light with an ideal semiconductor microcavity. We investigate photon statistics in different conditions and the presence of detuning and exciton-exciton interaction. We show that in the resonant interaction and absence of the exciton-exciton interaction, the state of the whole system can be considered as   coherent state. According to our results, it turns...

We theoretically study the efficiency of energy harvesting in linear exciton chains with an energy bias, where the initial excitation is taking place at the high-energy end of the chain and the energy is harvested (trapped) at the other end. The efficiency is characterized by means of the average time for the exciton to be trapped after the initial excitation. The exciton transport is treated a...

A phenomenological coupled exciton model is proposed in order to characterize optical excitations in extended dendrimers. An onsite exciton state is assigned at each phenyl rings and a nearest neighbor hopping integral which obeys the Gaussian distribution is considered between the exciton states. The decreasing optical excitation energy with respect to the dendrimer size indicates the presence...

Chalcogenide perovskites have emerged as non-toxic and stable photovoltaic materials, acting an alternative to lead halide hybrid having similar optoelectronic properties. In the present work, we report electronic optical properties of chalcogenide AZrS$_3$ (A=Ca, Sr, Ba) by using density functional theory (DFT) many-body perturbation (MBPT viz. G$_0$W$_0$ BSE). This study includes excitonic an...

We have developed a symmetry-based tight-binding (TB) method for calculating the electronic structure, exciton states and optical spectra in spherical semiconductor quantum dots (QD's). It is based on the semi-empirical sp^{3}s^{*} model, including thespin-orbit interaction. The TB parameters of the QD Hamiltonian are those used to reproduce the bulk semiconductor band structure. The surface da...

The photosynthetic apparatus of green sulfur bacteria, the chlorosome, is generally considered as a highly efficient natural light-harvesting system. The efficient exciton transport through chlorosomes toward the reaction centers originates from self-assembly of the bacteriochlorophyll molecules. The aim of the present work is to realize a long exciton diffusion length in an artificial light-ha...

We have succeeded in generating highly charged excitons in InAs self-assembled quantum dots by embedding the dots in a field-effect heterostructure. We discover an excitonic Coulomb blockage: over large regions of gate voltage, the exciton charge remains constant. We present here a summary of the emission properties of the charged excitons. INTRODUCTION An exciton is the elementary excitation i...

We show that optical two-dimensional (2D) spectroscopy can recover ultrafast heterogeneous dynamics of closely spaced delocalized exciton states from a molecular exciton manifold characterized by a single absorption band. The complete experimental third-order nonlinear optical response from room-temperature J-aggregates in liquid phase is reproduced for the first time with self-consistent Frenk...

The Hartree-Fock-Popov theory of interacting Bose particles is developed, for modeling exciton-polaritons in semiconductor microcavities undergoing Bose-Einstein condensation. A self-consistent treatment of the linear exciton-photon coupling and of the exciton nonlinearity provides a thermal equilibrium description of the collective excitation spectrum, of the polariton energy shifts and of the...

The dynamics of excitation energy transfer within the B850 ring of light harvesting complex 2 from Rhodobacter sphaeroides and between neighboring B850 rings is investigated by means of dissipative quantum mechanics. The assumption of Boltzmann populated donor states for the calculation of intercomplex excitation transfer rates by generalized Forster theory is shown to give accurate results sin...