We present data and initial results from VLT/X-Shooter emission-line spectroscopy of 96 galaxies selected by long γ-ray bursts (GRBs) at 0.1 < z < 3.6, the largest sample of GRB host spectra available to date. Most of our GRBs were detected by Swift and 76% are at 0.5 < z < 2.5 with a median zmed ∼ 1.6. Based on Balmer and/or forbidden lines of oxygen, nitrogen, and neon, we measure systemic re...