UNLABELLED All lanthanides have similar chemical properties regarding labeling. Therefore, radiolanthanides that have been used for therapy, such as (153)Sm and (177)Lu, might easily be replaced with other radiolanthanides. The aim of this work was to investigate the suitability of electron- and positron-emitting radiolanthanides for radionuclide therapy with reference to dosimetry and producti...

This thesis is composed of three Chapters. Chapter 1 is a preface that outlines the degree program and components of my thesis. Chapter 2 is the main body of the thesis; it is an investigation into pore pressures in the Auger basin and how they are related to fluid venting at the seafloor. I map the distribution of subsurface pressures in thick interconnected sand bodies that are present across...

Direct and inverse Auger scattering are amongst the primary processes that mediate the thermalization of hot carriers in semiconductors. These two processes involve the annihilation or generation of an electron-hole pair by exchanging energy with a third carrier, which is either accelerated or decelerated. Inverse Auger scattering is generally suppressed, as the decelerated carriers must have e...

As part of a project to compute improved atomic data for the spectral modeling of iron K lines, we report extensive calculations and comparisons of atomic data for K-vacancy states in Fe xxiv. The data sets include: (i) energy levels, line wavelengths, radiative and Auger rates; (ii) inner-shell electron impact excitation rates and (iii) fine structure inner-shell photoionization cross sections...

Auger decay spectra of CO subsequent to O 1s ionization with 549.85 eV photons, i.e. close to the top of the shape resonance, are presented. Their comparison with the normal Auger spectrum recorded at a photon energy well above the shape resonance reveals distinct features. In particular, in the energy region of the O 1s−1 → b15 and O 1s−1 → a16+ Auger transitions which are well known to consis...

In this Letter, we present nondegenerate ultrafast optical pump-probe studies of the carrier recombination dynamics in MoS2 monolayers. By tuning the probe to wavelengths much longer than the exciton line, we make the probe transmission sensitive to the total population of photoexcited electrons and holes. Our measurement reveals two distinct time scales over which the photoexcited electrons an...

Quantum-wire and quantum-box structures for narrow-gap materials with small effective masses, such as HgCdTe, can readily be fabricated using current lithographic techniques. In this article, we calculate the Auger-recombination carrier lifetimes in HgCdTe quantumwire and quantum-box structures, with band gaps in the 2-5 ,um wavelength range. Quantum confinement is generally believed to increas...

The fluorescence of colloidal CdSe/ZnS nanocrystals at room temperature exhibits a perfect antibunching under continuous or pulsed excitation. In this paper, we discuss the consequences of fluorescence properties of CdSe nanocrystals on the generation of single photons. In particular,we examine the role of Auger processes in the inhibition of multiexcitonic emission. We also discuss the relatio...

We propose a method to overcome Auger recombination in nanocrystal quantum dot lasers using cavity-enhanced spontaneous emission. We derive a numerical model for a laser composed of nanocrystal quantum dots coupled to optical nanocavities with small mode-volume. Using this model, we demonstrate that spontaneous emission enhancement of the biexciton transition lowers the lasing threshold by redu...

Radiative and Auger decay data have been calculated for modeling the K lines of the aluminum isonuclear sequence, from Al0 up to Al11+. Level energies, transition wavelengths, radiative transition probabilities, and radiative and Auger widths were determined using Cowan’s Hartree-Fock with relativistic corrections (HFR) method. Results are compared with data sets computed with the AUTOSTRUCTURE...